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Impact of Peak Material Volume of Polycrystalline CVD Diamond Coatings on Dry Friction Against Aluminum

MetadataDetails
Publication Date2020-05-07
JournalJOM
AuthorsM. Prieske
InstitutionsBremen Institute for Applied Beam Technology
Citations3
AnalysisFull AI Review Included

Technical Documentation: Optimized Polycrystalline CVD Diamond for Dry Tribology

Section titled “Technical Documentation: Optimized Polycrystalline CVD Diamond for Dry Tribology”

This document analyzes the findings of the research paper “Impact of Peak Material Volume of Polycrystalline CVD Diamond Coatings on Dry Friction Against Aluminum” and outlines how 6CCVD’s advanced MPCVD capabilities can meet and exceed the material requirements for high-performance dry forming and tribological applications.


The research successfully identified the critical surface topology parameter—Peak Material Volume (Vmp)—required for achieving ultra-low friction and wear rates in dry tribological contact between CVD diamond coatings and aluminum (EN AW 5083).

  • Critical Parameter Identified: The Peak Material Volume (Vmp) is the primary predictor for minimizing aluminum abrasion and achieving a low coefficient of friction (COF).
  • Performance Target: To minimize wear, the Vmp of the diamond coating surface must be maintained below 0.04 ml/m2.
  • Optimal Material: Microcrystalline Polycrystalline CVD Diamond (PCD) with subsequent mirror-polishing achieved the best results, demonstrating the lowest wear rate (4.5 x 10-9 mm3/Nm).
  • Friction Stability: The highly polished coating (CVDD 10.25p) exhibited the most constant and lowest COF (0.12-0.13) throughout the 99,900-cycle test.
  • Methodological Insight: Standard roughness parameters (Ra, Rq) were found to be insufficient for predicting tribological performance; precise control over the Vmp parameter is essential for engineering dry forming tools.
  • 6CCVD Value Proposition: 6CCVD specializes in producing high-purity PCD and SCD materials with custom post-processing, including mirror polishing (Ra < 1nm) necessary to achieve the required ultra-low Vmp values for competitive dry forming applications.

The following table summarizes the critical performance metrics and material parameters derived from the tribological investigation.

ParameterValueUnitContext
Target ApplicationDry Forming/ShapingN/AAluminum alloy EN AW 5083 counter body
Tribometer Test TypeOscillating Ball-on-PlateN/ADry contact, 99,900 cycles
Hertzian Contact Stress759MPaSimulating sheet metal forming conditions
Test Velocity50mm/sN/A
Critical Topology ParameterPeak Material Volume (Vmp)ml/m2Primary factor correlating to low wear and friction
Recommended Vmp Target< 0.04ml/m2Required to minimize aluminum wear rate
Lowest Achieved Vmp0.001ml/m2Achieved by mirror-polished CVDD 10.25p
Lowest Aluminum Wear Rate4.5 x 10-9mm3/NmAchieved by mirror-polished CVDD 10.25p
Lowest Friction Coefficient (COF)0.12 - 0.13N/AAchieved by mirror-polished CVDD 10.25p
Best Surface Roughness (Sa)0.02”mAchieved by mirror-polished CVDD 10.25p
Raman Quality Factor (Q)0.8 - 0.9N/AHigh quality factor (sp3 concentration)

The experiment utilized atmospheric pressure CVD diamond coatings deposited on K10 hard metal (WC-Co) substrates, followed by various surface post-treatments.

  1. Substrate Preparation: K10 hard metal discs (20.3 mm diameter) were etched using Murakami reagent and Caro’s reagent to remove cobalt and prepare the surface.
  2. Nucleation: Substrates were nucleated using a dispersion of 0.25 ”m to 0.50 ”m diamond powder in isopropanol via ultrasonic bath treatment.
  3. Deposition Method: Laser-based plasma CVD process at atmospheric pressure was used.
  4. Process Gas Parameters:
    • Total gas flow: 2 standard liters per minute (slm) of CH4/H2 mixture.
    • Argon plasma flame flow: 26 slm.
    • CH4/H2 ratio varied from 1% to 5%.
    • Deposition Temperature: Varied from 750 °C to 1050 °C.
    • Deposition Time: Varied from 12 minutes to 40 minutes.
  5. Post-Treatment: Coatings were either left untreated, mechanically polished (‘p’), or rubbed against another diamond layer (‘r’) to modify surface topology.
  6. Characterization: Surface roughness parameters (DIN EN ISO 25178) were measured using 3D laser microscopy. Diamond quality (sp3/sp2 ratio) was assessed via Micro-Raman spectroscopy (514 nm excitation).

The findings confirm that achieving optimal dry tribological performance requires precise control over diamond crystal size, film thickness, and, critically, post-deposition surface finishing to minimize the Peak Material Volume (Vmp). 6CCVD is uniquely positioned to supply materials engineered to these exact specifications.

To replicate or extend this research, 6CCVD recommends materials optimized for ultra-low roughness and high purity:

6CCVD Material RecommendationRationale & Application
High-Purity Polycrystalline CVD Diamond (PCD)Ideal for high-volume dry forming tools. We offer custom crystal sizes (microcrystalline, similar to the paper’s successful samples) and thicknesses up to 500 ”m, grown on various substrates (including WC-Co).
Optical Grade Single Crystal Diamond (SCD)For applications requiring the absolute lowest friction and wear. SCD offers superior initial surface quality and can be polished to Ra < 1 nm, ensuring Vmp values significantly lower than the 0.04 ml/m2 threshold.
Custom SubstratesWhile the paper used K10 hard metal, 6CCVD can deposit PCD/SCD films on custom substrates, including Si, Mo, W, or specialized ceramics, tailored to the client’s thermal and mechanical requirements.

The key to the paper’s success was the mirror-polished surface (CVDD 10.25p, Vmp = 0.001 ml/m2). 6CCVD offers industry-leading post-processing capabilities essential for achieving these results:

  • Ultra-Low Roughness Polishing: We guarantee surface roughness down to Ra < 5 nm for inch-size PCD plates and Ra < 1 nm for SCD, ensuring the Vmp parameter is minimized for optimal dry friction performance.
  • Custom Dimensions: While the paper used 20.3 mm discs, 6CCVD can supply PCD plates/wafers up to 125 mm in diameter, suitable for scaling up industrial dry forming processes.
  • Thickness Control: We provide precise thickness control for PCD coatings from 0.1 ”m up to 500 ”m, allowing engineers to optimize cost and performance based on expected tool life.
  • Metalization Services: If the application requires integration into complex tooling, 6CCVD offers in-house metalization capabilities (Au, Pt, Pd, Ti, W, Cu) for reliable bonding and electrical contact.

6CCVD’s in-house PhD team specializes in the relationship between MPCVD growth parameters, crystal morphology, and resulting surface topology. We can assist clients in defining the precise material specifications needed for similar Dry Metal Shaping and Forming projects:

  • Vmp Optimization: We consult on growth recipes and polishing techniques specifically targeting the required Vmp value (< 0.04 ml/m2) to ensure maximum tool life and minimum COF.
  • Quality Assurance: We provide detailed surface metrology reports, including 3D roughness parameters (Sa, Spk, Vmp, etc.) according to DIN EN ISO 25178, guaranteeing the material meets the critical tribological requirements identified in this research.

For custom specifications or material consultation, visit 6ccvd.com or contact our engineering team directly.

View Original Abstract

Abstract For economic and environmental reasons, dry forming is of increasing interest due to the shortening of process chains, cost savings and reduction of environmental pollution. The aim of these investigations is to examine to what extent chemical vapor deposited (CVD) diamond coatings are suitable for dry forming of aluminum and to identify the surface topology requirements for a low friction coefficient and low wear. Nine different surface topologies of CVD diamond coatings were tested in an oscillating ball-on-plate tribometer test against aluminum balls with a Hertzian contact stress of 759 MPa and 99,900 cycles. It could be concluded that the peak material volume (Vmp) of the diamond coating is the most important factor for achieving a low abrasion of aluminum as well as a low friction coefficient against aluminum. The Vmp should be smaller than 0.04 ml/m 2 . Microcrystalline CVD diamond with a post-treated surface has great potential for dry forming of aluminum.