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Preparing Multipartite Entangled Spin Qubits via Pauli Spin Blockade

MetadataDetails
Publication Date2020-02-26
JournalScientific Reports
AuthorsSinan Bugu, Fatih Özaydin, T. Ferrus, Tetsuo Kodera
InstitutionsHitachi (United Kingdom), Tokyo International University
Citations22
AnalysisFull AI Review Included

Preparing Multipartite Entangled Spin Qubits via Pauli Spin Blockade

Section titled “Preparing Multipartite Entangled Spin Qubits via Pauli Spin Blockade”

This technical documentation analyzes the proposed scheme for preparing large-scale multipartite entangled W states using electron spins in Double Quantum Dots (DQDs) via Pauli Spin Blockade (PSB).

  • Core Application: Preparation and manipulation of large-scale W states, a fundamental requirement for solid-state Quantum Information Processing (QIP).
  • Mechanism: Fusion of two smaller W states ($W_n$ and $W_m$) into a larger state ($W_{n+m-2}$) by injecting single electrons into a DQD and utilizing the presence or absence of Pauli Spin Blockade (PSB).
  • Key Advantage: The scheme is entirely based on solid-state electron spins and does not require complex optical cavities or photon assistance, simplifying technological implementation compared to previous proposals (e.g., NV centers requiring photonic qubits).
  • Material Requirements: Successful implementation relies critically on high-quality solid-state platforms (like diamond or silicon) that offer long electron spin coherence times (T2) and low noise environments.
  • Performance Enhancement: An improved setup utilizing a Toffoli + CNOT gate and an ancillary electron converts the probabilistic ‘failure case’ into a ‘successful case,’ significantly boosting the overall success rate.
  • Technological Readiness: The requirements for DQD fabrication, charge sensing (radio-frequency reflectometry), and logic gate implementation are based on currently available semiconductor and quantum dot technologies.

The following hard data points are extracted from the research paper, highlighting the critical performance metrics required for successful implementation.

ParameterValueUnitContext
Electron Spin Coherence Time (QDs)Few tens of”sMinimum required coherence time.
Electron Spin Coherence Time (DQDs)Tens ofmsDemonstrated coherence time in high-quality systems.
Electron Injection TimeFew hundreds ofpsTime required for electrons to tunnel into the DQD.
PSB Sensing Time (RF Reflectometry)FewnsRequired speed for fast, real-time detection.
PSB Sensing Time (Other Methods)Few hundreds ofnsAlternative sensing methods.
Minimum Fusible W State Sizen=3, m=3QubitsSmallest W state number demonstrated for fusion setup.
DQD Transport Cycle (PSB Regime)(0, 1) → (1, 1) → (0, 2) → (0, 1)N/ACharge configurations during the PSB cycle.
Ideal Fusion Fidelity(1-p)2 + p2N/AFidelity of the resulting $W_{n+m-2}$ state, where p is the probability of an electron spin flip during the process.

The proposed fusion scheme relies on precise control of electron tunneling and spin state detection within a DQD architecture.

  1. DQD Architecture Setup: A Double Quantum Dot (DQD) device is constructed, tunnel-coupled internally and to source/drain reservoirs, and capacitively coupled to side gates ($V_{sg1}$, $V_{sg2}$) for energy level tuning.
  2. Energy Level Tuning: The side gates are tuned to establish the Pauli Spin Blockade (PSB) regime, ensuring that inter-dot tunneling is blocked only when the two trapped electrons have parallel spins (Triplet state, T(1, 1)).
  3. Electron Injection: A single electron from each of the two initial W states ($W_A$ and $W_B$) is injected into the corresponding quantum dot (Dot 1 and Dot 2).
  4. PSB Sensing: A charge sensor (e.g., radio-frequency reflectometry or standard transport measurement) checks for the presence or absence of current flow through the DQD, which determines the spin configuration of the two injected electrons.
  5. Fusion Outcome Determination:
    • Absence of PSB (Success): Implies anti-parallel spins ($\downarrow\uparrow$ or $\uparrow\downarrow$), resulting in successful fusion to the larger $W_{n+m-2}$ state.
    • Presence of PSB (Recycle/Failure): Implies parallel spins ($\downarrow\downarrow$ or $\uparrow\uparrow$). The $\downarrow\downarrow$ case is recyclable, while the $\uparrow\uparrow$ case is a failure, requiring advanced logic gates to mitigate.
  6. Enhanced Fusion Scheme: To improve success rate, an ancillary spin-down electron and logic gates (Toffoli + CNOT) are placed before the DQD, converting the catastrophic $\uparrow\uparrow$ failure case into a successful fusion outcome.

The research highlights the critical need for high-quality, low-noise solid-state platforms to achieve the required millisecond-scale coherence times for electron spin qubits. 6CCVD’s expertise in MPCVD diamond provides the ideal material solution to meet and exceed these stringent requirements.

To replicate or extend this research, particularly in the context of NV centers or high-coherence spin qubits, 6CCVD recommends the following materials:

  • Optical Grade Single Crystal Diamond (SCD): Essential for achieving the longest possible spin coherence times (T2). SCD offers the lowest concentration of impurities (like Nitrogen) and defects, minimizing charge noise and maximizing qubit fidelity, which is paramount for stable PSB sensing and gate operations.
  • High-Purity Polycrystalline Diamond (PCD): Suitable for large-area quantum circuits or substrates where the active DQD region is localized. Our PCD offers excellent thermal management and mechanical stability.
  • Boron-Doped Diamond (BDD): Can be utilized for creating conductive layers or electrodes necessary for the DQD side gates ($V_{sg1}$, $V_{sg2}$) or charge sensor components, offering robust, chemically inert contacts.

The fabrication of DQD devices requires precise material engineering, etching, and metal deposition. 6CCVD offers comprehensive customization capabilities directly supporting this research:

Research Requirement6CCVD Customization Capability
Substrate Quality & Noise ReductionUltra-Low Roughness Polishing: SCD wafers are polished to an atomic-scale roughness (Ra < 1nm), and inch-size PCD to Ra < 5nm. This minimizes surface defects that contribute to charge noise, crucial for stable PSB sensing.
Gate Electrode IntegrationCustom Metalization: We provide in-house deposition of critical gate metals (Au, Pt, Pd, Ti, W, Cu) required for forming the DQD side gates and tunnel barriers, ensuring robust electrical contact and integration.
Scalable CircuitryCustom Dimensions: We supply SCD plates up to 500”m thick and PCD wafers up to 125mm in diameter, facilitating the development of scalable, multi-DQD quantum circuits necessary for large W state generation.
Defect EngineeringControlled NV Creation: For researchers focusing on NV-center-based spin qubits (as mentioned in the paper’s context), 6CCVD offers controlled nitrogen incorporation and post-growth processing to optimize NV density and location.

The successful implementation of this DQD-based fusion scheme requires careful material selection to mitigate leakage processes caused by Spin-Orbit Coupling (SOC) and Hyperfine Interaction (HFI).

  • Material Selection for QIP: 6CCVD’s in-house PhD team specializes in material optimization for quantum applications. We can assist researchers in selecting the optimal diamond grade (SCD vs. PCD) and orientation to minimize intrinsic defects and maximize electron spin coherence for similar Solid-State Quantum Dot projects.
  • Global Logistics: We ensure reliable, global delivery of custom diamond materials, with DDU (Delivered Duty Unpaid) as the default shipping method and DDP (Delivered Duty Paid) available upon request.

For custom specifications or material consultation, visit 6ccvd.com or contact our engineering team directly.

View Original Abstract

Abstract Preparing large-scale multi-partite entangled states of quantum bits in each physical form such as photons, atoms or electrons for each specific application area is a fundamental issue in quantum science and technologies. Here, we propose a setup based on Pauli spin blockade (PSB) for the preparation of large-scale W states of electrons in a double quantum dot (DQD). Within the proposed scheme, two W states of n and m electrons respectively can be fused by allowing each W state to transfer a single electron to each quantum dot. The presence or absence of PSB then determines whether the two states have fused or not, leading to the creation of a W state of n + m − 2 electrons in the successful case. Contrary to previous works based on quantum dots or nitrogen-vacancy centers in diamond, our proposal does not require any photon assistance. Therefore the ‘complex’ integration and tuning of an optical cavity is not a necessary prerequisite. We also show how to improve the success rate in our setup. Because requirements are based on currently available technology and well-known sensing techniques, our scheme can directly contribute to the advances in quantum technologies and, in particular in solid state systems.