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Periodically driven three-level systems

MetadataDetails
Publication Date2016-09-01
JournalPhysical review. B./Physical review. B
AuthorsM. B. Kenmoe, Lukong Cornelius Fai
InstitutionsUniversité de Dschang
Citations18
AnalysisFull AI Review Included

Technical Documentation & Analysis: Periodically Driven Three-Level Systems in Diamond

Section titled “Technical Documentation & Analysis: Periodically Driven Three-Level Systems in Diamond”

This document analyzes the provided research paper, focusing on the application of diamond-based Three-Level Systems (ThLS, or qutrits) for Quantum Information Processing (QIP). The analysis is structured to provide key technical specifications and directly connect the material requirements to 6CCVD’s advanced MPCVD diamond capabilities, driving sales to researchers and engineers in the quantum technology sector.


The research provides a comprehensive theoretical framework for controlling Three-Level Systems (ThLS, or qutrits) using periodic electromagnetic drives, with direct application to the Nitrogen Vacancy Center (NVC) in diamond.

  • Qutrit Control in Diamond: The study confirms that the NVC spin-1 system in diamond serves as an ideal solid-state qutrit platform, offering robustness and longer coherence times compared to two-level systems (qubits).
  • LZSM Interferometry: The dynamics are characterized by cascaded SU(3) Landau-Zener-StĂŒckelberg-Majorana (LZSM) interferometers, demonstrating complex coherent control pathways.
  • Adiabatic and Non-Adiabatic Regimes: Analytical and numerical solutions validate the system dynamics across weak and strong longitudinal and transverse driving limits, providing recipes for fast (non-adiabatic) and slow (adiabatic) quantum manipulation.
  • Coherent Destruction of Tunneling (CDT): The work identifies conditions under which the longitudinal drive can be tuned to the zeroes of the Bessel function, inhibiting population transfer (destructive interference).
  • Material Requirement: Successful implementation relies entirely on high-quality, low-defect Single Crystal Diamond (SCD) to host the NVC centers and maintain the required long coherence times.
  • 6CCVD Value: 6CCVD specializes in the high-purity MPCVD SCD necessary for replicating and scaling these NVC-based quantum experiments.

The following hard data points and parameters were extracted from the analysis of the Three-Level System (ThLS) dynamics, specifically applied to the NVC in diamond.

ParameterValueUnitContext
System TypeSpin-1N/AThree-Level System (ThLS) / Qutrit
Host PlatformNitrogen Vacancy Center (NVC)N/ASolid-state quantum computing candidate
Uniaxial Anisotropy (D)$2\pi \times 2.88$GHzZero-field splitting term in NVC ground state
Longitudinal Drive Amplitude ($A/2\pi$)4.6GHzExample for numerical simulation (MW signal)
Transverse Drive Amplitude ($A_f/2\pi$)0.6GHzExample for numerical simulation (RF signal)
Measurement Time Scale7.96nsTypical time scale for population evolution
Key PhenomenonSU(3) LZSM OscillationsN/AInterference patterns demonstrating multiple transitions
Required Material PurityUltra-low NitrogenN/AEssential for maximizing NVC coherence time
Required Surface QualityRa < 1nmNecessary for optical access (confocal microscopy)

The experimental dynamics of the ThLS were analyzed using a combination of theoretical modeling and numerical simulation, focusing on the Hamiltonian $H(t)$ and its time-dependent Schrödinger equation (TDSE).

  1. Hamiltonian Definition: The system was modeled using the Hamiltonian $H(t) = H_Q(t) + H_{drive}(t) + D(S^z)^2$, incorporating longitudinal AC drive ($A \cos(\omega t) S^z$), transverse AC drive ($A_f \cos(\omega_f t) S^x$), and uniaxial anisotropy ($D(S^z)^2$).
  2. Analytical Approximations: The TDSE was solved analytically using two primary approximations: the transverse drive limits ($A_f \ll \omega$ and $A_f \gg \omega$) and the longitudinal drive limits ($A \ll \omega$ and $A \gg \omega$).
  3. Adiabatic Basis Transformation: For the strong transverse drive limit, a general adiabatic theory was constructed by transforming the system into the composite Hilbert space generated by the time-dependent basis vectors (eigenstates of the perturbed Hamiltonian).
  4. Numerical Validation: Analytical results for population probabilities ($P_{\kappa’ \to \kappa}(t)$) were rigorously tested against exact numerical solutions of the TDSE, confirming the validity of the approximations across various regimes.
  5. NVC Application: The theoretical framework was directly applied to the NVC in diamond, using known parameters (e.g., $D = 2\pi \times 2.88 \text{GHz}$) and comparing results to existing MW/RF experimental data.

The successful replication and scaling of this NVC-based qutrit research fundamentally depend on the quality and customization of the diamond substrate. 6CCVD provides the necessary high-specification MPCVD diamond materials and engineering services.

Research Requirement6CCVD Material RecommendationTechnical Justification
NVC Host MaterialOptical Grade Single Crystal Diamond (SCD)Ultra-low nitrogen concentration (< 1 ppb) is critical to minimize decoherence and maximize the intrinsic spin coherence time ($T_2^*$) of the NVC centers, enabling robust QIP.
High-Density Qutrit ArraysPolycrystalline Diamond (PCD) SubstratesFor scaling up to large arrays or integrating complex microwave circuitry, our PCD wafers (up to 125mm diameter) offer a cost-effective, large-area platform with excellent thermal management.
Gate Electrodes/CircuitryBoron-Doped Diamond (BDD)BDD films can be used as conductive layers for integrated microwave or radio-frequency transmission lines necessary to apply the periodic longitudinal and transverse drives ($A, A_f$).

The complexity of quantum experiments often requires materials tailored beyond standard specifications. 6CCVD offers full customization to meet the precise needs of NVC research:

  • Custom Dimensions and Thickness: While the paper implies small samples, scaling NVC arrays requires larger substrates. 6CCVD provides SCD and PCD plates/wafers up to 125mm in diameter. SCD thickness ranges from 0.1”m to 500”m, and substrates up to 10mm are available for robust mechanical mounting.
  • Ultra-Precision Polishing: NVC experiments rely on optical access (confocal microscopy, optical pumping). We guarantee Ra < 1nm polishing on SCD and Ra < 5nm on inch-size PCD, ensuring minimal surface scattering losses.
  • Integrated Metalization: The application of AC drives (MW/RF) requires precise electrode placement. 6CCVD offers in-house metalization services, including deposition of Ti/Pt/Au, Pd, W, and Cu, allowing researchers to define custom gate geometries directly onto the diamond surface.

6CCVD’s in-house PhD team provides authoritative professional support, assisting researchers in material selection and optimization for complex quantum projects. We understand the critical relationship between diamond purity, crystal orientation, and NVC performance. We can assist with material selection for similar NVC/ThLS Coherent Control projects, ensuring the diamond substrate meets the stringent requirements for long coherence times and high optical quality.

Call to Action: For custom specifications or material consultation regarding NVC platforms, LZSM interferometry, or other diamond-based quantum projects, visit 6ccvd.com or contact our engineering team directly. We offer global shipping (DDU default, DDP available) to ensure timely delivery of your critical materials.

View Original Abstract

We study the dynamics of a three-level system (ThLS) sinusoidally driven in\nboth longitudinal and transverse directions and in the presence of a uniaxial\nanisotropy $D$ entering the generic Hamiltonian through the zero-energy\nsplitting term $D(S^{z})^{2}$ where $S^{z}$ is the projection of the spin\nvector along the quantization direction. As a consequence of the addition of\nthis term, the order of the symmetry group of the Hamiltonian is increased by a\nunit and we observe a sequence of cascaded $SU(3)$\nLandau-Zener-St\“uckelberg-Majorana (LZSM) interferometers. The study is\ncarried out by analytically and numerically calculating the probabilities of\nnon-adiabatic and adiabatic evolutions. For non-adiabatic evolutions, two main\napproximations based on the weak and strong driving limits are discussed by\ncomparing the characteristic frequency of the longitudinal drive with the\namplitudes of driven fields. For each of the cases discussed, our analytical\nresults quite well reproduce the gross temporal profile of the exact numerical\nprobabilities. This allows us to check the range of validity of analytical\nresults and confirm our assumptions. For adiabatic evolutions, a general theory\nis constructed allowing for the description of adiabatic passages in arbitrary\nThLSs in which direct transitions between states with extremal spin projections\nare forbidden. A compact formula for adiabatic evolutions is derived and\nnumerically tested for some illustrative cases. Interference patterns\ndemonstrating multiple LZSM transitions are reported. Applications of our\nresults to the Nitrogen Vacancy Center (NVC) in diamond are discussed.\n