Skip to content

Quantum Zeno and Zeno-like effects in nitrogen vacancy centers

MetadataDetails
Publication Date2015-12-01
JournalScientific Reports
AuthorsJing Qiu, Yangyang Wang, Zhang‐qi Yin, Mei Zhang, Qing Ai
InstitutionsTsinghua University, Beijing Normal University
Citations17
AnalysisFull AI Review Included

Technical Documentation & Analysis: Quantum Zeno Effects in NV Centers

Section titled “Technical Documentation & Analysis: Quantum Zeno Effects in NV Centers”

This research successfully demonstrates the Quantum Zeno Effect (QZE) and Quantum Zeno-Like Effect (QZLE) in a solid-state system, utilizing a Nitrogen Vacancy (NV) center coupled to a proximal 13C nuclear spin in diamond. This work validates the use of MPCVD diamond as a robust platform for advanced quantum information processing (QIP) and sensing applications.

  • Core Achievement: Realization of QZE and QZLE in a 13C nuclear spin by controlling the electron spin of an adjacent NV center.
  • Material Requirement: The experiment relies on the exceptional spin coherence properties of the NV center, necessitating ultra-high purity, low-strain Single Crystal Diamond (SCD).
  • Key Performance Metric: Demonstrated long nuclear spin coherence time (T2n ~1 second) at room temperature (300 K), enabling the execution of approximately 2 x 104 measurement cycles within the total experiment time (100 ms).
  • Methodology: QZE/QZLE is achieved through finite-frequency, imperfect measurements modulated by microwave pulses (Rabi frequency < 10 MHz) and subsequent electron spin initialization via 532 nm optical pumping.
  • 6CCVD Value Proposition: 6CCVD provides the necessary foundation—high-quality, custom-engineered SCD substrates—critical for achieving and extending these long coherence times and integrating complex microwave and optical control systems.

The following parameters and performance metrics were extracted from the analysis of the NV center system used to demonstrate QZE/QZLE:

ParameterValueUnitContext
Material SystemNV Center in DiamondN/ASolid-state qubit platform
Zero-Field Splitting (D)2.87GHzGround state 3A spin-triplet
Operating TemperatureRoom TemperatureK300 K
Nuclear Spin Coherence (T2n)~1second13C nuclear spin
Electron Spin Coherence (T2e)58”sElectron spin dephasing time
Total Experiment Time (T)100msRestricted to T << T2n
Single Cycle Duration (τ)~5”sSum of free evolution (∆tf) and measurement (∆tm)
Measurement Pulse Duration (∆tm)~2”sMicrowave pulse width
Optical Pumping Pulse~140ns532 nm light for electron spin initialization
Maximum Rabi Frequency (Ω)< 10MHzLimited by 13C hyperfine coupling (130 MHz)
Applied Magnetic Field (Bz)< 200GRequired for secular approximation validity
Hyperfine Coupling (Azz)130MHz13C in the first coordination shell

The demonstration of QZE and QZLE relies on a precise, repetitive cycle of free evolution, microwave-induced transition, and optical initialization.

  1. Material Preparation: Utilization of a negatively-charged NV center (S=1) in diamond, coupled to a nearest-neighbor 13C nuclear spin (I=1/2).
  2. Initial State Preparation: Electron spin is initialized into the ground state |0> via circulatory optical excitation-emission (532 nm light pulse, ~140 ns duration). The nuclear spin is prepared in an arbitrary state.
  3. Free Evolution (∆tf): The system evolves freely under the Hamiltonian HF for a time interval ∆tf.
  4. Measurement Pulse (∆tm): A microwave pulse (duration ~2 ”s) is applied, driving the transition between the electronic spin states |0,↑> and |-1,↑>. The driving frequency is set to be resonant with this transition while being largely detuned from the |0,↓> and |-1,↓> transition.
  5. Repolarization/Decoupling: After measurement, the electron spin is re-initialized to |0> via optical pumping. Crucially, the 13C nuclear spin is designed to be well isolated and unperturbed during this optical process.
  6. QZE/QZLE Observation: The conventional QZE and QZLE are observed by modulating key parameters (Rabi frequency Ω, magnetic field Bz, and cycle times ∆tf, ∆tm) to control the eigenvalues of the nuclear spin state evolution operator.

The success of QZE/QZLE experiments hinges on the quality and precise engineering of the diamond substrate. 6CCVD is uniquely positioned to supply the foundational materials and customization services required to replicate and advance this research.

To achieve the long coherence times (T2n ~1s) and high fidelity required for QIP, researchers need diamond with extremely low nitrogen and other impurity concentrations.

Material Requirement6CCVD SolutionTechnical Advantage
Ultra-High Purity SubstrateOptical Grade Single Crystal Diamond (SCD)SCD grown via MPCVD ensures minimal defects and strain, maximizing T2e and T2n coherence times at room temperature.
Isotopic Control (13C)Custom Isotope-Enriched SCDWhile the paper uses naturally occurring 13C, 6CCVD can supply SCD grown using precursors enriched in 13C (to increase qubit density) or highly depleted in 13C (12C > 99.995%) to further suppress nuclear spin bath decoherence and extend T2e.
Boron Doping (Optional Extension)Boron-Doped Diamond (BDD)For applications requiring conductive diamond electrodes or integrated sensors, 6CCVD offers BDD films with controlled doping levels.

The integration of microwave and optical control systems demands precise material dimensions and surface quality. 6CCVD offers full customization to meet complex experimental setups:

  • Custom Dimensions: 6CCVD supplies plates and wafers up to 125 mm (PCD) and custom SCD sizes. We can provide substrates up to 10 mm thick, suitable for high-power microwave integration and robust mounting.
  • Precision Polishing: The experiment relies on 532 nm optical pumping. 6CCVD guarantees Ra < 1 nm polishing for SCD surfaces, ensuring minimal scattering loss and optimal optical access for high-fidelity initialization and readout.
  • Integrated Metalization: The control scheme requires precise microwave delivery. 6CCVD offers in-house metalization services (Au, Pt, Pd, Ti, W, Cu) for creating custom microwave striplines, coplanar waveguides, or contact pads directly on the diamond surface, facilitating seamless integration of the Rabi frequency control mechanism.
  • Laser Cutting and Shaping: We provide custom laser cutting services to shape substrates for specific geometries required by microwave resonators or cryostat mounts.

The successful implementation of QZE/QZLE requires careful tuning of the magnetic field (Bz < 200 G) and precise control over the hyperfine interaction (Azz).

6CCVD’s in-house PhD team specializes in the physics of NV centers and MPCVD growth parameters. We offer expert consultation on:

  • Material Selection: Assisting researchers in selecting the optimal isotopic purity and nitrogen concentration (P1 centers) to balance qubit density and coherence time for similar Quantum Zeno Effect projects.
  • Interface Optimization: Advising on surface termination and metalization schemes to minimize microwave loss and maximize coupling efficiency for Rabi frequency control (Ω).

Call to Action: For custom specifications or material consultation, visit 6ccvd.com or contact our engineering team directly.