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Lithium Extraction from Salt Lakes - Maximizing Efficiency with BDD Electrodes in Electrochemical Oxidation and TOC Evaporation Performance

MetadataDetails
Publication Date2025-06-01
JournalJournal of Salt Lake Research
AuthorsZhimin He, Cong Zhao, Zhiyi Liao, Jinsong He, Shiyi Xiao
AnalysisFull AI Review Included

BDD Electrode Optimization for High-TOC Brine Treatment in Lithium Extraction

Section titled “BDD Electrode Optimization for High-TOC Brine Treatment in Lithium Extraction”

Technical Documentation & Sales Analysis for 6CCVD

This document analyzes the research paper, “Lithium Extraction from Salt Lakes: Maximizing Efficiency with BDD Electrodes in Electrochemical Oxidation and TOC Evaporation Performance,” to highlight the critical role of high-quality Boron-Doped Diamond (BDD) electrodes and to position 6CCVD’s advanced MPCVD diamond materials as the optimal solution for industrial replication and scale-up.


The research validates Boron-Doped Diamond (BDD) electrochemical oxidation (BDD-EO) as a superior method for degrading high Total Organic Carbon (TOC) concentrations in aggressive lithium extraction brines.

  • Core Achievement: BDD-EO successfully reduced TOC from an initial 1,550 mg/L to 66.8 mg/L in 24 hours under optimal conditions.
  • Optimal Parameters: The most efficient single-step BDD-EO parameters were identified as 60 °C reaction temperature and 70 mA/cm2 current density.
  • Energy Optimization: A hybrid process combining macroporous resin adsorption, short-duration BDD-EO (4 hours), and activated carbon adsorption achieved a final TOC of 52 mg/L, significantly reducing overall energy consumption.
  • Material Validation: The study confirms BDD’s exceptional stability, wide electrochemical potential window, and resistance to corrosion, making it ideal for treating complex, high-salt, high-acid industrial wastewater.
  • Oxidant Findings: The addition of H₂O₂ was found to be detrimental, inhibiting the direct electron transfer oxidation pathway crucial for efficient TOC removal in this specific system.
  • Industrial Relevance: The findings provide a practical, cost-effective pathway for stabilizing evaporation mother liquor, ensuring reliable downstream processing (evaporation, crystallization, and electrolysis).

The following hard data points were extracted from the research detailing the performance of the BDD electrochemical oxidation system.

ParameterValueUnitContext
Initial TOC Concentration1,550mg/LRaw evaporation mother liquor
Optimal Reaction Temperature60°CFor BDD Electrochemical Oxidation
Optimal Current Density (J)70mA/cm2Balance of efficiency and energy cost
TOC Reduction (24h BDD-EO only)1,550 → 66.8mg/LMaximum single-step removal
TOC Reduction (Optimized Hybrid Process)1,550 → 52mg/LResin + 4h BDD-EO + Activated Carbon
BDD-EO Time (Optimized Hybrid)4hReduced time for energy efficiency
Resin Adsorption Flow Rate2BV/hXDA-1 Macroporous Resin
Activated Carbon Adsorption Time6hC1 Activated Carbon (Static Adsorption)
H₂O₂ EffectNegativeN/AInhibits direct oxidation pathway (R → (R)+ + e)

The experiment focused on optimizing the BDD-EO process parameters and integrating adsorption techniques to achieve high TOC removal efficiency while minimizing energy consumption.

  1. Electrode Material: Boron-Doped Diamond (BDD) electrodes were utilized in a dedicated electrochemical oxidation device (SDN-BDD100-10001).
  2. Raw Material: Evaporation mother liquor sourced from a large chemical enterprise, characterized by high TOC (1,550 mg/L), low pH (3.95), and high concentrations of Li+, Na+, and Cl-.
  3. Parameter Optimization: Systematic investigation of four key variables:
    • Reaction Temperature (20 °C to 80 °C).
    • Current Density (50 mA/cm2 to 80 mA/cm2).
    • Electrolysis Time (1 h to 24 h).
    • Oxidant Addition (H₂O₂ concentration 0 vol% to 4 vol%).
  4. TOC Analysis: Total Organic Carbon was measured using a Shimadzu TOC-4200 analyzer via combustion oxidation—non-dispersive infrared absorption, adhering to the HJ501-2009 standard.
  5. Optimized Hybrid Strategy: Based on energy consumption analysis, a three-stage, cost-effective process was implemented:
    • Stage 1 (Pre-treatment): Dynamic adsorption using XDA-1 macroporous resin (2 BV/h, 25 °C).
    • Stage 2 (Core Treatment): BDD Electrochemical Oxidation (4 hours at 60 °C, 70 mA/cm2).
    • Stage 3 (Polishing): Static adsorption using C1 activated carbon (6 hours at 25 °C).

This research confirms the industrial viability of BDD electrodes for demanding environmental and resource recovery applications. 6CCVD is uniquely positioned to supply the high-performance BDD materials required to replicate and scale this technology globally.

To replicate or extend this research into pilot or industrial scale, engineers require robust, high-conductivity BDD material.

6CCVD MaterialSpecificationApplication Relevance
Heavy Boron-Doped Diamond (BDD)Polycrystalline (PCD) or Single Crystal (SCD)Provides the wide electrochemical window and stability necessary for efficient TOC degradation in high-salt brines.
High-Purity PCD SubstratesUp to 125mm diameterIdeal for large-area electrode fabrication required for industrial-scale lithium extraction facilities.
Custom Metalized BDDTi/Pt/Au, W/Au, or Cu contactsEnsures low-resistance electrical contact and corrosion protection in aggressive electrochemical reactors.

The study utilized materials relevant to a “large chemical enterprise,” implying the need for large, durable electrodes. 6CCVD’s manufacturing capabilities directly address these industrial requirements:

  • Large-Area Electrodes: We offer Polycrystalline Diamond (PCD) plates up to 125mm in diameter, enabling the fabrication of large-scale electrochemical cells necessary for high-volume brine processing.
  • Custom Thickness: We supply BDD layers in thicknesses ranging from 0.1 ”m to 500 ”m, allowing engineers to optimize material usage based on expected electrode lifetime and current density requirements.
  • Advanced Metalization: The long-term stability of the BDD electrode relies heavily on robust electrical contacts. 6CCVD provides in-house, multi-layer metalization (e.g., Ti/Pt/Au) tailored to withstand the high temperatures (60 °C) and corrosive environment of the mother liquor.
  • Precision Polishing: While BDD is often used in an as-grown state for electrochemistry, we offer polishing services (Ra < 5nm for PCD) to ensure uniform surface morphology and consistent current distribution across large plates, maximizing reactor efficiency.

6CCVD’s in-house PhD team specializes in the material science of MPCVD diamond for electrochemical and sensor applications. We offer consultation services to assist clients in:

  • Material Selection: Determining the optimal boron doping level and substrate type (SCD vs. PCD) for specific Lithium Brine TOC Degradation projects.
  • Electrode Design: Advising on optimal electrode geometry, thickness, and metal contact placement for maximizing current efficiency (mA/cm2) and minimizing energy consumption (kWh·kg-1).
  • Global Logistics: Providing reliable, DDU or DDP global shipping for time-sensitive industrial projects.

For custom specifications or material consultation, visit 6ccvd.com or contact our engineering team directly.