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Quantum magnetometry of transient signals with a time resolution of 1.1 nanoseconds

MetadataDetails
Publication Date2025-01-18
JournalNature Communications
AuthorsKonstantin Herb, Laura A. VÓ§lker, John M. Abendroth, Nicholas Meinhardt, Laura van Schie
InstitutionsETH Zurich
Citations5
AnalysisFull AI Review Included

Technical Documentation & Analysis: Ultra-Fast Quantum Magnetometry

Section titled “Technical Documentation & Analysis: Ultra-Fast Quantum Magnetometry”

Reference: K. Herb et al., “Quantum magnetometry of transient signals with a time resolution of 1.1 nanoseconds,” Nature Communications 16:822 (2025).


This research demonstrates a significant advancement in quantum sensing, achieving nanosecond-scale time resolution for magnetic field detection using a single Nitrogen-Vacancy (NV) center in diamond. This capability is critical for rapidly evolving fields such as spintronics and nanoscale device metrology.

  • Record Temporal Resolution: Achieved a best-effort time resolution of 1.1 ns and an instantaneous bandwidth of 0.9 GHz, an order of magnitude faster than previous targeted approaches.
  • Core Application: Enables time-resolved investigation of ultra-fast magnetic phenomena, including magnetization reversals and domain wall propagation in magnetic nanostructures.
  • Material Foundation: Success relies on high-quality, electronic-grade Single Crystal Diamond (SCD) substrates integrated with nanopillar waveguide arrays and optimized Co-Planar Waveguide (CPW) antennas.
  • High-Frequency Performance: Demonstrated high Rabi frequencies (Ω/2π ≈ 125 MHz, corresponding to Bmw ≈ 6.3 mT) essential for short-pulse quantum control sequences.
  • Precision Timing: Achieved a Time-of-Flight (ToF) precision better than 20 ps, demonstrating exceptional timing stability for transient signal analysis.
  • Future Scalability: The methodology is scalable toward picosecond resolution, requiring advanced diamond integration and ultra-low loss microwave delivery systems.

The following hard data points were extracted from the experimental results and methodology sections:

ParameterValueUnitContext
Best-Effort Time Resolution (tmin)1.1nsAchieved using α = 45° spin rotation angle
Instantaneous Frequency Bandwidth (ΩBw)0.9GHzCorresponding to 1.1 ns resolution
Time-of-Flight (ToF) Precision< 20psAbsolute timing error
Maximum Rabi Frequency (Ω/2π)125MHzAchieved with Bmw ≈ 6.3 mT
Nominal Sensitivity (Bmin)35”T/HzCalculated for α = π/2, τ = 2 ns
Bias Magnetic Field (B0)36mTApplied axially to isolate ms=0 to ms=-1 transition
NV Center Implantation Energy5keV15N+ ion implantation
NV Center Implantation Fluence109cm-2Used for single NV creation
Annealing Temperature1200°CRequired for NV activation
CPW 3 dB Bandwidthca. 7.5GHzCoplanar Waveguide antenna design
CPW Center Conductor Width20”mNarrowed core section for field concentration

The experimental success hinges on precise material engineering and advanced quantum control techniques:

  1. Substrate Selection and Preparation: Experiments utilized electronic-grade Single Crystal Diamond (SCD) with natural isotope composition, ensuring high material purity necessary for long NV coherence times.
  2. NV Center Creation: NV centers were created via 15N+ ion implantation (5 keV energy, 109 cm-2 fluence), followed by high-vacuum annealing at 1200 °C for 4 hours to activate the defects.
  3. Photonic Structure Fabrication: Nanopillar waveguide arrays were fabricated on membrane samples using electron-beam lithography (EBL) and Reactive Ion Etching (RIE) to enhance photon collection efficiency.
  4. Microwave Delivery Integration: A broad-band (ca. 8 GHz) Co-Planar Waveguide (CPW) antenna, fabricated by patterning gold onto a quartz coverslip, was positioned within ca. 25 ”m of the NV center array to maximize the microwave field amplitude (Bmw).
  5. Quantum Control Protocol: A pump-probe scheme employing equivalent-time sampling and a speed-optimized two-pulse sequence (P1-P2) was used to sample the transient magnetic field B(t).
  6. Signal Deconvolution: Time resolution was optimized post-measurement using numerical Wiener deconvolution, which accounts for pulse distortions and the full S=1 nature of the NV spin system (including non-linear effects and Bloch-Siegert shifts).

The demonstrated research requires ultra-high quality diamond substrates and advanced fabrication capabilities—core competencies of 6CCVD. We provide the necessary materials and engineering support to replicate, extend, and industrialize this cutting-edge quantum magnetometry technique.

To achieve the long coherence times and low noise floor required for this nanosecond sensing protocol, the research necessitates the highest quality diamond.

  • Optical Grade Single Crystal Diamond (SCD): 6CCVD offers electronic-grade SCD plates with extremely low nitrogen and defect concentrations, crucial for maximizing the NV center coherence time (T2) and minimizing baseline noise (Bmin ≈ 35 ”T/Hz).
  • Custom Thicknesses: We supply SCD wafers ranging from 0.1 ”m up to 500 ”m, allowing researchers to optimize the thickness for subsequent nanopillar fabrication and membrane processing (RIE etching).

The integration of NV centers with complex microwave structures (CPW) and photonic elements (nanopillars) demands precise material processing and integration services, which 6CCVD provides in-house.

Research Requirement6CCVD CapabilityTechnical Advantage
Substrate GeometryCustom dimensions for plates/wafers up to 125 mm (PCD) and custom SCD sizes.Supports precise integration into high-frequency microwave setups and custom chip carriers.
Surface QualityUltra-low roughness polishing: Ra < 1 nm (SCD).Essential for high-fidelity electron-beam lithography (EBL) and subsequent RIE etching required for nanopillar waveguide arrays.
Microwave IntegrationInternal metalization services: Au, Ti, Pt, Pd, W, Cu.Enables direct fabrication of high-performance CPW antennas (e.g., Ti/Au stacks) onto the diamond surface, ensuring precise impedance matching and minimizing absorptive losses necessary for high Rabi frequencies (>125 MHz).
Advanced StructuresLaser cutting and shaping services.Facilitates the creation of complex geometries and precise alignment features required for optical and microwave coupling.

The transition to picosecond resolution requires achieving Rabi frequencies exceeding 1 GHz, demanding specialized material selection and integration strategies to manage high-frequency effects (e.g., Bloch-Siegert shifts, non-resonant transitions).

  • Application Expertise: 6CCVD’s in-house PhD team specializes in material selection and optimization for similar Spintronics, Nanoscale Device Metrology, and Quantum Sensing projects.
  • High-Frequency Optimization: We consult on material specifications (e.g., low-loss dielectric properties) necessary for achieving the ultra-high Rabi frequencies (440 MHz to >1 GHz) required for next-generation picosecond sensing protocols.
  • Global Logistics: We offer reliable global shipping (DDU default, DDP available) to ensure rapid delivery of custom-engineered diamond solutions worldwide.

For custom specifications or material consultation, visit 6ccvd.com or contact our engineering team directly.