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Effect of freeze-thaw cycles on water permeability of sand mixtures with nanoclay

MetadataDetails
Publication Date2024-03-29
JournalARCTIC AND SUBARCTIC NATURAL RESOURCES
AuthorsА Л ĐĐ”ĐČĐ·ĐŸŃ€ĐŸĐČ, Yu. V. Saenko, A. M Shiranov, Sergey Churkin
InstitutionsNorthern (Arctic) Federal University
AnalysisFull AI Review Included

Technical Documentation & Analysis: High-Precision Geotechnical Testing Components

Section titled “Technical Documentation & Analysis: High-Precision Geotechnical Testing Components”

This document analyzes the research paper “Effect of freeze-thaw cycles on water permeability of sand mixtures with nanoclay” (Nevzorov et al., 2024) to identify critical material requirements for high-precision geotechnical testing equipment, aligning these needs with 6CCVD’s advanced MPCVD diamond solutions.


This research highlights the necessity for extremely stable, wear-resistant, and thermally robust components in geotechnical testing apparatus designed for Arctic and sub-Arctic conditions. 6CCVD specializes in providing the foundational materials required for such high-precision instrumentation.

  • Application Focus: Investigating the degradation of waste isolation liners (sand/nanoclay mixtures) under cyclic freeze-thaw conditions.
  • Methodological Demand: The custom-built, patented apparatus requires components capable of maintaining dimensional stability and precision under simultaneous mechanical load (up to 12 kPa) and extreme temperature gradients (from 1.5 °C to -6 °C).
  • Precision Requirement: Accurate measurement of frost heave (1.9-4.0 mm residual deformation) and minute changes in hydraulic conductivity (k increased by 1.2-4.7 times) necessitates ultra-stable sensor platforms and low-friction interfaces.
  • 6CCVD Value Proposition: MPCVD Single Crystal Diamond (SCD) and Polycrystalline Diamond (PCD) are the ideal materials for critical components (e.g., sensor substrates, high-wear stamps, flow meter parts) due to their unmatched hardness, thermal stability, and customizable electrical properties.
  • Customization: 6CCVD offers custom-sized SCD/PCD plates up to 125 mm, precision polishing (Ra < 1 nm for SCD), and custom metalization schemes (e.g., Ti/Pt/Au) essential for integrating diamond components into complex sensor systems.

The following hard data points extracted from the research paper define the operational environment and performance metrics that necessitate high-performance materials for the testing apparatus.

ParameterValueUnitContext
Sample Height100mmStandard sample dimension (Diameter 70 mm)
External Load (Low Clay)2kPaApplied load for 4% clay mixtures
External Load (High Clay)12kPaApplied load for 8% clay mixtures (equivalent to 0.7 m soil layer)
Freezing Temperature (Chamber)-(5
6)°CStandard operating temperature
Thawing Temperature (Water Bath)1
1.5°CWater bath temperature for thawing
Frost Heave (4% Clay, 2 kPa)10.0-16.4%Relative deformation of the sample
Residual Deformation (4% Clay, 5 cycles)2.1-4.0mmTotal permanent deformation after 5 cycles
Hydraulic Conductivity Increase (4% Clay)2.0-4.7TimesIncrease factor (kf/ko) after 5 cycles
Hydraulic Conductivity Increase (8% Clay)1.2-2.0TimesIncrease factor (kf/ko) after 5 cycles
Number of Cycles5CyclesStandard test duration
Freezing Front Velocity10-19mm/dayControlled rate of freezing front movement

The experiment utilized a specialized, patented laboratory setup to precisely control and measure the effects of cyclic freezing and thawing on saturated soil samples.

  1. Apparatus Configuration: Experiments were conducted using a custom-built apparatus (Patent RU 2 586 271 C1) consisting of four devices housed in a freezer chamber (T = -(5
6) °C).
  2. Sample Preparation: Mixtures of four types of sand and saponite nanoclay (4% or 8% clay content by mass) were compacted to a density coefficient of 0.94-0.96. Samples were 100 mm high and 70 mm in diameter.
  3. Load Application: External loads (2 kPa or 12 kPa) were applied via a metallic stamp (5) placed on the upper surface of the sample.
  4. Temperature Control & Measurement: The water level in the surrounding container was gradually lowered (10 mm/day) to control the freezing front velocity. Thermistors were embedded at 25 mm, 50 mm, and 75 mm depths, and under the stamp, to monitor temperature gradients.
  5. Cyclic Testing: Samples underwent five complete freeze-thaw cycles. Thawing was achieved by raising the water bath temperature to 1.5 °C, followed by raising the chamber temperature to +20 °C for 4 hours to ensure complete thawing.
  6. Permeability Measurement: Hydraulic conductivity (k) was measured before the first cycle (ko) and after the fifth cycle (kf) using a constant head method, with water supplied from below via a pump with a built-in flow meter.

The high-precision, multi-cycle testing environment described in this research demands materials that offer superior stability, wear resistance, and thermal management—qualities inherent to MPCVD diamond. 6CCVD provides the necessary custom diamond components to enhance the reliability and longevity of geotechnical testing equipment.

Applicable Materials for High-Precision Geotechnical Apparatus

Section titled “Applicable Materials for High-Precision Geotechnical Apparatus”
Component Requirement6CCVD Material RecommendationRationale & Benefit
High-Load Stamps/Plates (5)Polycrystalline Diamond (PCD) PlatesExtreme hardness and wear resistance prevent deformation or scratching under high external loads (12 kPa) and repeated contact with abrasive sand/clay mixtures. PCD ensures consistent load distribution over 5+ cycles.
Sensor Substrates (Displacement/Pressure)Optical Grade Single Crystal Diamond (SCD)Unmatched thermal conductivity (up to 2200 W/mK) ensures rapid heat dissipation for sensitive electronics (e.g., displacement sensors, thermistor readouts). SCD’s low coefficient of thermal expansion (CTE) guarantees dimensional stability across the required T gradient (1.5 °C to -6 °C).
Flow Meter/Valve ComponentsHeavy Boron Doped PCD (BDD) or SCDBDD offers chemical inertness and electrochemical stability, ideal for components exposed to water and potential contaminants (filtrate). Diamond’s hardness ensures long-term calibration stability in flow restrictors or pump heads.
Thermal Isolation/ManagementHigh-Purity SCD SubstratesCan be engineered as highly efficient heat sinks or, conversely, as stable thermal barriers, crucial for maintaining the precise, controlled temperature gradient required for accurate freezing front velocity (10 mm/day).

Customization Potential for Research Replication and Extension

Section titled “Customization Potential for Research Replication and Extension”

The complexity of the patented apparatus (RU 2 586 271 C1) necessitates highly customized components. 6CCVD’s in-house capabilities directly address these needs:

  • Custom Dimensions and Geometry: The research used 70 mm diameter samples. 6CCVD can supply PCD and SCD plates up to 125 mm in diameter, allowing for scaling up the testing apparatus or creating custom-shaped stamps and restrictor plates (4, 5).
  • Precision Polishing: For critical interfaces, 6CCVD offers SCD polishing to Ra < 1 nm and PCD polishing to Ra < 5 nm (for inch-size plates). This low roughness minimizes friction and ensures accurate displacement readings from the stamp (5) and displacement sensor (6).
  • Advanced Metalization: Integrating diamond into sensor systems requires robust electrical contacts. 6CCVD offers internal metalization capabilities including Au, Pt, Pd, Ti, W, and Cu, enabling the creation of custom sensor platforms or heating elements directly on the diamond substrate.
  • Thickness Control: We provide SCD and PCD materials with precise thickness control, ranging from 0.1 ”m to 500 ”m for thin films, and robust substrates up to 10 mm for structural components like load stamps.

6CCVD’s in-house PhD team possesses deep expertise in diamond material science and its application in extreme environments. We can assist researchers in selecting the optimal diamond grade (SCD, PCD, or BDD) and geometry to maximize the precision and lifespan of equipment used in similar Geotechnical Freeze-Thaw Testing projects.

Call to Action: For custom specifications or material consultation regarding high-stability components for extreme environmental testing, visit 6ccvd.com or contact our engineering team directly.

View Original Abstract

The mixtures of sands and nanoclays are used to isolate municipal and industrial solid wastes. Compared with natural clayey soils, these mixtures are characterized by homogeneous composition, workability, and low compressibility. This study investigated the eïŹ€ect of freeze-thaw cycles on their permeability. The mixtures of four sands and a saponite clay suspension generated by diamond ore processing were studied. The mixtures were prepared on the basis of 4 % and 8 % clay from sand weight. The tests were performed using an apparatus consisting of four devices for measuring frost heave and permeability, which were placed in containers with water. The water level was decreased gradually to ensure sample freezing or increased to ensure sample thawing. The frost heave of the mixtures with 4 % clay was 10.0-16.4 % under an external load of 2 kPa, and the ïŹve freeze-thaw cycles resulted in an increase in the hydraulic conductivity by 2.0-4.7 times. The mixtures with 8 % clay were tested under a load of 12 kPa, because of their high frost susceptibility. The hydraulic conductivity increased by approximately the same value as in the ïŹrst case, i.e., by 1.2-2.0 times. The experiments have shown that the examined mixtures are suitable for isolating wastes. However, to eliminate the above eïŹ€ect, a waterproof liner should be covered with inert soil, which would reduce the depth of frost penetration and apply the load on it.