Skip to content

Enhancing quantum sensing performance by optimizing the concentration and dephasing time of the NV ensemble in CVD-diamond

MetadataDetails
Publication Date2022-12-15
JournalOptical Materials Express
AuthorsSixian Wang, Guodong Bian, Pengcheng Fan, Mingxin Li, Bo Li
InstitutionsEast China Normal University
Citations4

The negatively charged nitrogenāˆ’vacancy (NV āˆ’ ) center ensembles in diamonds offer enormous potential for developing integrated sensors with an improved signal-to-noise ratio (SNR) and high sensitivity. However, the preparation and treatment of diamond samples with suitable NV āˆ’ concentrations and dephasing time have remained challenging. This work provided insight into the NV āˆ’ center formation mechanism and reconstruction via a comprehensive analysis of the concentration and dephasing time of a set of diamond samples treated by various parameters. By varying the electron irradiation dose and subsequent annealing duration, the conversion rate of nitrogen to NV āˆ’ is up to 18.45%, and the corresponding maximum NV āˆ’ concentration is 3.69 ppm. The dephasing time for all samples varies around 300 ns. The nitrogen-related NV āˆ’ center ensemble dephasing rate per unit density is 146.4 (ppmĀ·ms) āˆ’1 , indicating that the treatment did not substantially alter the paramagnetic spin environment around the NV āˆ’ center. This study not only offers support to exquisite sensitivities of NV-based sensors but also provides valuable experience for the preparation of unique properties of synthetic diamonds.