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Quantum Simulation for Three-Dimensional Chiral Topological Insulator

MetadataDetails
Publication Date2020-07-10
JournalPhysical Review Letters
AuthorsWentao Ji, Lin Zhang, Mengqi Wang, Long Zhang, Yuhang Guo
InstitutionsUniversity of Chinese Academy of Sciences, Peking University
Citations54
AnalysisFull AI Review Included

6CCVD Technical Documentation: MPCVD Diamond for Quantum Simulation

Section titled “6CCVD Technical Documentation: MPCVD Diamond for Quantum Simulation”

Research Paper Analyzed: Quantum simulation for three-dimensional chiral topological insulator (Ji et al., arXiv:2002.11352v2)

This document analyzes the material requirements and experimental methodology of the referenced research, focusing on how 6CCVD’s specialized MPCVD diamond products—particularly high-purity Single Crystal Diamond (SCD)—can enable the replication, scaling, and extension of solid-state quantum simulation platforms.


  • Platform Validation: The research successfully utilized a solid-state spin system based on the Nitrogen-Vacancy (NV) center in diamond to simulate a previously unrealized 3D chiral topological insulator.
  • Material Requirement: The experiment critically relies on ultra-high quality Single Crystal Diamond (SCD) to host the NV center, providing the necessary low-noise environment for the two-qubit system (electron spin and intrinsic 14N nuclear spin).
  • Core Achievement: Demonstrated a complete study of both bulk and surface topological physics using dynamical bulk-surface correspondence in momentum space, a technique highly suited for quantum simulators.
  • Symmetry Verification: Chiral symmetry protection was verified by measuring dynamical spin textures on Band Inversion Surfaces (BISs), confirming the robustness of the topological phase.
  • Dynamical Transition: Identified an emergent dynamical topological transition by varying the quantum quench depth, opening new avenues for studying topological quantum phases.
  • Operating Conditions: The NV center system proved robust, performing complex quantum simulation protocols at room temperature, highlighting the stability of diamond-based quantum devices.

The following hard data points were extracted from the experimental setup and results, detailing the physical parameters required for the NV center quantum simulator:

ParameterValueUnitContext
Simulation PlatformNV Center in DiamondN/ATwo-qubit system (Electron S=1, 14N I=1)
Diamond Orientation[111]N/ARequired for alignment with applied magnetic field
Operating TemperatureRoom TemperatureN/AExperiment performed on a home-built confocal setup
Electronic Zero-Field Splitting (D)2.87GHzIntrinsic NV property
Nuclear Quadrupolar Interaction (Q)-4.95MHzIntrinsic NV property
Hyperfine Interaction (A)-2.16MHzIntrinsic NV property
Applied Magnetic Field514GApplied along the NV symmetry axis
Electron Zeeman Splitting (we)1439MHzResulting from applied field
Nuclear Zeeman Splitting (wn)154kHzResulting from applied field
Critical Quench Depth (mc)≈ 2.7toN/APoint of emergent dynamical topological transition
Maximum Simulation Time (tsim)2”sUsed for time-averaged spin polarization measurements

The experiment utilized a sequence of microwave (MW) and radio-frequency (RF) pulses combined with optical readout to realize and measure the complex 3D chiral topological Hamiltonian (H3D) within the NV center system.

  1. Material Preparation: A [111] oriented Single Crystal Diamond (SCD) hosting an NV center was used, coupled with a solid immersion lens (SIL) for efficient optical access.
  2. Qubit Initialization: The system was initialized to the |00> state (corresponding to the electron and nuclear spin ground states) using a 532 nm green laser pulse.
  3. Hamiltonian Mapping: The target Hamiltonian H3D(k) was mapped onto the NV center’s effective Hamiltonian (Heff) by controlling the parameters ($\theta$, $\phi$, $\Omega_{mw}$) via MW and RF pulses.
  4. Quench Dynamics: The system underwent quantum quenches by preparing the initial state (fully or partially polarized along $\gamma_i$ axes) followed by evolution under H3D for a defined time $t$.
  5. Topological Measurement (Bulk-Surface Correspondence): The Band Inversion Surfaces (BISs) were identified as the momenta where time-averaged spin polarizations $\langle \gamma_i(\mathbf{k}) \rangle$ vanish.
  6. Symmetry Protection Measurement: Dynamical spin-texture fields $\mathbf{g}(\mathbf{k})$ were measured on the BISs to characterize the 3D winding number ($W$) and verify chiral symmetry protection.
  7. Topological Charge Detection: Topological charges were characterized by the dynamical field $\mathbf{\Theta}(\mathbf{k})$, measured via a series of quenches along different axes, demonstrating the bulk topology and the emergent dynamical transition.
  8. Readout: Spin polarizations were measured by transforming the desired component to the $z$ basis using MW/RF pulses, followed by photoluminescence (PL) photon counting.

The successful implementation of this 3D quantum simulation relies fundamentally on the quality and precise engineering of the diamond host material. 6CCVD is uniquely positioned to supply the next generation of SCD substrates required for scaling and advancing NV-based quantum technologies.

To replicate or extend this research, the highest quality diamond is essential for maximizing coherence times (T2) and minimizing spectral diffusion.

Application Requirement6CCVD Recommended MaterialKey Specification
NV Center HostOptical Grade Single Crystal Diamond (SCD)Ultra-low nitrogen concentration (< 1 ppb) for long T2 coherence times.
Orientation ControlCustom [111] SCD SubstratesPrecise orientation control (e.g., < 0.5°) is critical for aligning the NV axis with external magnetic fields (514 G).
High-Density IntegrationHigh-Purity Polycrystalline Diamond (PCD)Available for large-area sensor arrays or heat spreading, with wafers up to 125 mm diameter.
Integrated Qubit ControlBoron-Doped Diamond (BDD)Available for creating integrated micro-electrodes or waveguides adjacent to the NV layer.

The experiment utilized a specific [111] orientation and required high-quality optical surfaces for confocal microscopy and solid immersion lens (SIL) integration. 6CCVD offers comprehensive customization services to meet these advanced engineering needs:

  • Precision Polishing: We guarantee ultra-smooth surfaces essential for low-loss optical coupling (e.g., SIL integration). Our SCD polishing achieves surface roughness Ra < 1 nm.
  • Custom Dimensions and Thickness: We provide SCD plates with thicknesses ranging from 0.1 ”m up to 500 ”m, allowing researchers to optimize the depth of the NV layer relative to the surface.
  • Advanced Metalization: For future experiments requiring integrated microwave or RF control lines (as used in the quench and readout steps), 6CCVD offers in-house metalization services, including Ti/Pt/Au, W, Pd, and Cu deposition, patterned to custom specifications.
  • Substrate Engineering: We can supply SCD substrates up to 10 mm thick for robust mechanical and thermal support in complex cryogenic or high-field setups.

6CCVD’s in-house team of PhD material scientists and quantum engineers specializes in the growth and characterization of diamond optimized for quantum applications. We offer consultation on:

  • NV Creation Optimization: Assisting researchers in selecting the optimal diamond growth parameters (e.g., nitrogen doping levels, post-growth annealing) to achieve the desired NV density and spin coherence properties for similar Topological Quantum Simulation projects.
  • Integration Strategy: Providing technical guidance on bonding, laser cutting, and surface preparation necessary for integrating diamond chips into complex quantum setups (e.g., microwave resonators, optical cavities).

For custom specifications or material consultation, visit 6ccvd.com or contact our engineering team directly.

View Original Abstract

Quantum simulation, as a state-of-the-art technique, provides a powerful way to explore topological quantum phases beyond natural limits. Nevertheless, it is usually hard to simulate both the bulk and surface topological physics at the same time to reveal their correspondence. Here we build up a quantum simulator using nitrogen-vacancy center to investigate a three-dimensional (3D) chiral topological insulator, and demonstrate the study of both the bulk and surface topological physics by quantum quenches. First, a dynamical bulk-surface correspondence in momentum space is observed, showing that the bulk topology of the 3D phase uniquely corresponds to the nontrivial quench dynamics emerging on 2D momentum hypersurfaces called band inversion surfaces (BISs). This is the momentum-space counterpart of the bulk-boundary correspondence in real space. Further, the symmetry protection of the 3D chiral phase is uncovered by measuring dynamical spin textures on BISs, which exhibit perfect (broken) topology when the chiral symmetry is preserved (broken). Finally, we measure the topological charges to characterize directly the bulk topology and identify an emergent dynamical topological transition when varying the quenches from deep to shallow regimes. This work demonstrates how a full study of topological phases can be achieved in quantum simulators.