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Single-Spin Magnetomechanics with Levitated Micromagnets

MetadataDetails
Publication Date2020-04-24
JournalPhysical Review Letters
AuthorsJan Gieseler, Aaron Kabcenell, Emma Rosenfeld, J. D. Schaefer, Arthur Safira
InstitutionsHarvard University, Max Planck Institute of Quantum Optics
Citations90
AnalysisFull AI Review Included

Technical Documentation & Analysis: Single-Spin Magnetomechanics

Section titled “Technical Documentation & Analysis: Single-Spin Magnetomechanics”

This document analyzes the requirements and achievements detailed in the research paper “Single-Spin Magnetomechanics with Levitated Micromagnets” and maps them directly to 6CCVD’s advanced MPCVD diamond capabilities, focusing on material solutions for quantum sensing and nanomechanics.


This research demonstrates a robust platform for achieving strong spin-mechanical coupling, utilizing a levitated micro-magnet interacting with a Nitrogen Vacancy (NV) center hosted in a diamond slab.

  • Core Achievement: Successful demonstration of direct magnetic coupling between a massive mechanical oscillator (micro-magnet) and an individual NV spin qubit in diamond.
  • Performance Metrics: Achieved mechanical quality factors (Q) around 106 and trapping frequencies in the kHz range, setting a new benchmark for magnetized resonators.
  • Material Requirement: The system relies critically on high-quality diamond to host NV centers, providing long spin coherence times ($T_2$) and enabling optical initialization/readout.
  • Coupling Strength: Measured spin-mechanical coupling strength ($\lambda_g$) of 48 $\pm$ 2 mHz, confirming the thermal character of the driven mode.
  • Future Potential: The platform is projected to reach the ultra-strong coupling regime ($\lambda_g > \omega_j$) necessary for ground-state cooling, quantum network realization, and ultra-sensitive metrology (magnetometers, accelerometers).
  • 6CCVD Value Proposition: 6CCVD provides the necessary high-purity Single Crystal Diamond (SCD) substrates, custom dimensions, and ultra-low roughness polishing (Ra < 1 nm) required to maximize NV coherence and mechanical Q-factors for next-generation experiments.

The following hard data points were extracted from the research paper, highlighting the critical parameters achieved or required for this spin-mechanics platform.

ParameterValueUnitContext
Mechanical Quality Factor (Q)$\sim 10^6$DimensionlessAchieved Q-factor for translational modes.
Target Q-Factor for Coherence$10^8$DimensionlessRequired for achieving cooperativity $C > 1$ at 4 K.
Maximum Trapping Frequency ($f_{max}$)25.2 $\pm$ 3.3kHzCenter-of-mass mode for the smaller particle ($a_2$).
Magnet Radius ($a_3$)15.1 $\pm$ 0.1”mParticle used for NV coupling experiment.
NV Implantation Depth ($d_{impl}$)$\sim 40$nmDepth below the diamond surface.
Superconductor Critical Temperature ($T_c$)$\sim 90$KYBCO film used for flux trapping levitation.
Operating Pressure$\lt 10^{-5}$mBarRequired to eliminate air damping as a dissipation source.
Measured Spin-Mechanical Coupling ($\lambda_g$)48 $\pm$ 2mHzCoupling strength achieved between magnet and NV center.
NV Zero Point Motion ($x_{zp}$)24 $\pm$ 1fmCalculated zero point motion of the magnet.
Target Minimum Gap ($d_{min}$)0.25”mConservative gap required for maximum gradient coupling.

The experiment relies on precise material integration and cryogenic control to achieve stable levitation and strong coupling.

  1. Diamond Preparation: A diamond slab was prepared with negatively charged NV centers implanted $\sim 40$ nm below the surface, providing the electronic spin qubit.
  2. Superconductor Setup: A Type-II Yttrium Barium Copper Oxide (YBCO) superconductor film was positioned below the diamond slab.
  3. Controlled Cooldown: The YBCO film was cooled below its critical temperature ($T_c \approx 90$ K) while controlling the distance ($h_{cool}$) between the magnet and the superconductor to freeze in the magnetic flux.
  4. 3D Trapping: Stable three-dimensional levitation of the hard micro-magnet was achieved by reducing the distance between the magnet and the now superconducting YBCO film.
  5. Motion Detection: Magnet center-of-mass motion was observed using a long working distance microscope and fast camera, allowing for calculation of Power Spectral Densities (PSD) and Q-factors via ringdown measurements.
  6. Spin Readout: The magnet’s motion was sensed by monitoring the optically detected magnetic resonance (ODMR) spectrum of the NV center, which shifts due to the magnetic field gradient generated by the moving magnet.

6CCVD is uniquely positioned to supply the advanced diamond materials and fabrication services required to replicate this foundational research and push the system toward the ultra-strong coupling regime ($C > 1$).

To maximize the spin coherence time ($T_2$) and minimize mechanical dissipation, the highest quality diamond is essential.

Research Requirement6CCVD Material SolutionTechnical Advantage
NV Host MaterialOptical Grade Single Crystal Diamond (SCD)Ultra-low nitrogen content (PPM level) and minimal strain, crucial for maximizing NV $T_2$ coherence times at cryogenic temperatures.
High-Frequency ResonatorsThin SCD Membranes (0.1 ”m - 50 ”m)Custom thickness control for fabricating high-Q mechanical resonators or thin slabs for close proximity to the levitated magnet.
Future Sensing/ElectrodesBoron-Doped Diamond (BDD)Available for integration as conductive electrodes or heating elements, if required for future electrical control or sensing schemes.

The paper highlights the need for precise geometries (slabs, pockets) and minimal separation ($d_{min} = 0.25$ ”m) to enhance coupling. 6CCVD provides the necessary fabrication precision.

  • Custom Dimensions and Thickness: 6CCVD supplies SCD plates and wafers up to 125 mm in size. We offer precise thickness control for SCD (0.1 ”m to 500 ”m) and substrates (up to 10 mm), allowing researchers to optimize the diamond slab geometry relative to the levitation pocket depth ($\sim 80$ ”m used in the paper).
  • Ultra-Smooth Polishing: Achieving the projected Q-factor of $10^8$ requires minimizing surface defects and strain. 6CCVD guarantees ultra-smooth polishing with surface roughness Ra < 1 nm for SCD, ensuring optimal optical access and reduced surface-related decoherence for the NV centers.
  • Precision Fabrication: We offer advanced laser cutting and etching services to create custom geometries, ensuring precise alignment of the diamond slab relative to the magnet pocket and the superconductor.
  • Custom Metalization: For future experiments requiring electrical control or integration with superconducting circuits (e.g., SQUID detection mentioned in the paper), 6CCVD offers in-house metalization capabilities, including Ti, Pt, Au, Pd, W, and Cu deposition.

6CCVD’s in-house PhD team specializes in optimizing MPCVD diamond for quantum applications. We offer comprehensive support for projects focused on Spin-Mechanical Coupling and Quantum Metrology.

  • Material Selection Consultation: Assistance in selecting the optimal diamond grade (purity, doping) and orientation for maximizing NV center performance and minimizing mechanical losses.
  • Integration Guidance: Technical advice on preparing diamond surfaces for implantation, bonding, and integration with cryogenic systems and Type-II superconductors (YBCO).
  • Global Logistics: We ensure reliable, global shipping (DDU default, DDP available) to deliver sensitive materials directly to research facilities worldwide.

For custom specifications or material consultation, visit 6ccvd.com or contact our engineering team directly.

View Original Abstract

We demonstrate a new mechanical transduction platform for individual spin qubits. In our approach, single micromagnets are trapped using a type-II superconductor in proximity of spin qubits, enabling direct magnetic coupling between the two systems. Controlling the distance between the magnet and the superconductor during cooldown, we demonstrate three-dimensional trapping with quality factors around 1×10^{6} and kHz trapping frequencies. We further exploit the large magnetic moment to mass ratio of this mechanical oscillator to couple its motion to the spin degrees of freedom of an individual nitrogen vacancy center in diamond. Our approach provides a new path towards interfacing individual spin qubits with mechanical motion for testing quantum mechanics with mesoscopic objects, realization of quantum networks, and ultrasensitive metrology.