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Bloch–Siegert oscillations in the Rabi model with an amplitude-modulated driving field

MetadataDetails
Publication Date2019-10-23
JournalLaser Physics
AuthorsA. P. Saiko, S.A. MARKEVICH, R. Fedaruk, A. P. Saiko, S.A. MARKEVICH
InstitutionsUniversity of Szczecin, National Academy of Sciences of Belarus
Citations7
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Technical Analysis and Documentation for 6CCVD

Section titled “Technical Analysis and Documentation for 6CCVD”

The analyzed research details a novel method for the direct observation and measurement of the Bloch-Siegert (BS) shift ($\omega^{\text{BS}}$) in two-level quantum systems operating in the ultrastrong coupling (USC) regime, using an amplitude-modulated microwave field. This technique is specifically proposed for implementation using Nitrogen Vacancy (NV) centers in diamond, directly linking the findings to 6CCVD’s core MPCVD Single Crystal Diamond (SCD) capabilities.

  • Core Achievement: Demonstration of a technique to isolate the Bloch-Siegert oscillation ($\omega^{\text{BS}}$) from complex multiphoton coherent dynamics.
  • Physical Mechanism: Destructive interference of multiple photon processes at the Rabi resonance forces the RWA Rabi frequency ($\Omega$) to vanish, leaving the dynamics dominated by the BS shift.
  • Material Focus: The experiment relies on the coherent spin dynamics of the NV center in solid-state Single Crystal Diamond (SCD).
  • Spectral Signature: The key observable is the transformation of the Fourier spectrum response from a series of triplets into characteristic doublets, where the splitting is precisely $2\omega^{\text{BS}}$.
  • Operational Regime: Requires operation in the ultrastrong coupling regime, characterized by a coupling constant $A \text{cos} \theta / \omega \approx 0.57$.
  • Application Relevance: Provides a critical new technique for precision measurement and coherent control of spin qubits, highly valuable for quantum information processing and quantum sensing applications.

The following parameters were utilized in the theoretical model, simulating conditions achievable in NV center diamond experiments:

ParameterValueUnitContext
Low-Frequency Modulation ($\omega$) / 2$\pi$10.44MHzPrimary driving field modulation frequency
High-Frequency Detuning ($\Delta_{\text{x}}$) / 2$\pi$10MHzField relative detuning parameter
Qubit Detuning ($\Delta_{\text{z}}$) / 2$\pi$3MHzEnergy transition parameter
Coherence Time ($\tau$)4µsPhenomenological decay time used for Fourier analysis
Ultrastrong Coupling Constant ($A \text{cos} \theta / \omega$)$\approx 0.57$-Regime necessary for significant non-RWA effects
Rabi Resonance Condition ($A^{*} / \omega$)2.00-Low-frequency amplitude value where $\Omega=0$
Bloch-Siegert Shift ($\omega_{\nu}$) / 2$\pi$20.9MHzExample maximum shift observed in the second triplet
Observable Splitting (Doublet)$2\omega^{\text{BS}}$MHzUsed for direct measurement of the BS shift

The theoretical framework proposes an advanced coherent spectroscopy technique based on the precise manipulation of energy levels in the ultrastrong coupling regime:

  1. Qubit System Selection: Utilizing a two-level spin qubit system (e.g., NV center $|0\rangle$ and $|-1\rangle$ sublevels) initially prepared in the ground state $|0\rangle$.
  2. Bichromatic Driving Field: Excitation using an amplitude-modulated microwave field $V(t)$, comprising high- and low-frequency components ($\omega_{1}$ and $\omega$) to induce complex coherent dynamics.
  3. Frame Transformations: Applying sequential rotating frame transformations and canonical transformations to simplify the interaction Hamiltonian ($H \rightarrow H_{1} \rightarrow H_{2}$).
  4. Effective Hamiltonian Derivation: Employing the Bogoliubov averaging method (up to the second order) to construct a time-independent effective Hamiltonian ($H_{\text{eff}}$), accounting for non-secular (non-RWA) terms.
  5. Rabi Resonance Tuning: Precisely tuning the low-frequency amplitude ($A$) such that the RWA Rabi frequency ($\Omega$) vanishes due to destructive interference of multiphoton processes ($A = A^{*}$, where $J_{1}(a)=0$).
  6. Direct Observation: Monitoring the time-resolved evolution of the ground state population $P_{|0\rangle}(t)$, which, at the tuned resonance, exhibits pure Bloch-Siegert oscillations ($\Omega^{*} = \omega^{\text{BS}}$).
  7. Spectral Analysis: Analyzing the Fourier spectrum of $P_{|0\rangle}(t)$ to confirm the transformation of multiphoton triplets ($n\omega \pm \Omega^*$) into doublets ($n\omega \pm \omega^{\text{BS}}$), allowing the direct determination of $2\omega^{\text{BS}}$.

The replication and advancement of this cutting-edge quantum research—focused on NV centers and ultrastrong coupling—depend critically on the quality and customization of the underlying diamond material. 6CCVD provides the necessary engineered MPCVD diamond solutions to support this highly technical field.

Requirement from Paper (NV Research)6CCVD Material/SolutionTechnical Specification Match
High Coherence Time (4 µs stated)Optical Grade Single Crystal Diamond (SCD)Our high-purity SCD is optimized for low residual nitrogen concentration (< 1 ppb possible) to maximize $T_{2}$ coherence and facilitate optimal NV formation/isolation.
Qubit Integration & Device FabricationCustom Dimensions & Thickness ControlWe offer SCD materials in thicknesses ranging from 0.1 µm to 500 µm. Crucial for thin film quantum devices and integrated photonics.
Surface Criticality (NV Proximity)Ultra-Smooth PolishingOur proprietary polishing capabilities guarantee surface roughness of Ra < 1 nm for SCD wafers, essential for minimizing surface noise and preserving qubit coherence near the surface.
Microwave Delivery StructureIn-House Custom Metalization ServicesWe provide internal metalization layering including Au, Pt, Pd, Ti, W, and Cu. This is vital for depositing co-planar waveguides or antennas required to deliver the amplitude-modulated microwave field (USC regime).
Reproducibility & ScalabilityLarge Format CapabilityWhile NV research often uses smaller samples, 6CCVD can produce high-quality PCD plates up to 125 mm, ensuring scalability of future quantum integrated circuits.

To replicate or extend this research utilizing NV centers for direct Bloch-Siegert shift measurement, the following 6CCVD material is essential:

  • Optical Grade Single Crystal Diamond (SCD): Required due to the need for high lattice purity and low defects/impurities to support long coherence times ($\tau$). The quality must support controlled creation and manipulation of NV centers.

The utilization of an amplitude-modulated microwave field often requires integration with patterned metal structures on the diamond surface.

  • 6CCVD offers extensive custom metalization capabilities, allowing researchers to define complex Ti/Pt/Au or other multilayer stacks for efficient microwave delivery into the USC regime.
  • We provide precision laser cutting and shaping to deliver custom geometry plates and wafers required for mounting in specialized cryogenic or microwave spectroscopy setups.

Understanding the complex interplay between qubit dynamics (Rabi oscillations, Bloch-Siegert effects) and material properties (nitrogen concentration, defect density) is crucial. 6CCVD’s in-house PhD-level engineering team specializes in MPCVD diamond properties for quantum applications. We can assist researchers with material selection, thickness optimization, and surface preparation specifications specifically tailored for similar Solid-State Spin Qubit Coherent Control projects.


For custom specifications or material consultation, visit 6ccvd.com or contact our engineering team directly.

View Original Abstract

We study the coherent dynamics of a qubit excited by an amplitude-modulated\nelectromagnetic field under the Rabi resonance when the frequency of the\nlow-frequency modulation field matches the Rabi frequency in the high-frequency\nfield. Due to destructive interference of multiple photon processes at the\nultrastrong coupling between the qubit and the low-frequency driving field,\nRabi oscillations result exclusively from the Bloch-Siegert effect. It is\ndirectly observed in the time-resolved coherent dynamics as the Bloch-Siegert\noscillation. In this case, triplets in Fourier spectra of the coherent response\nare transformed into doublets with the splitting between the lines equal to\ntwice the Bloch-Siegert shift. These unusual properties are demonstrated in\nconditions of experiments with a nitrogen vacancy center in diamond.\n