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Dependence of high density nitrogen-vacancy center ensemble coherence on electron irradiation doses and annealing time

MetadataDetails
Publication Date2017-11-02
JournalJournal of Physics D Applied Physics
AuthorsChen Zhang, Heng Yuan, N Zhang, Lixia Xu, Bo Li
InstitutionsBeihang University, Institute of Semiconductors
Citations39

Negatively charged nitrogen-vacancy (NVāˆ’) center ensembles in diamond have proved to have great potential for use in highly sensitive, small-package solid-state quantum sensors. One way to improve sensitivity is to produce a high-density NVāˆ’ center ensemble on a large scale with a long coherence lifetime. In this work, the NVāˆ’ center ensemble is prepared in type-Ib diamond using high energy electron irradiation and annealing, and the transverse relaxation time of the ensemble—T2—was systematically investigated as a function of the irradiation electron dose and annealing time. Dynamical decoupling sequences were used to characterize T2. To overcome the problem of low signal-to-noise ratio in T2 measurement, a coupled strip lines waveguide was used to synchronously manipulate NVāˆ’ centers along three directions to improve fluorescence signal contrast. Finally, NVāˆ’ center ensembles with a high concentration of roughly 1015 mmāˆ’3 were manipulated within a ~10 µs coherence time. By applying a multi-coupled strip-lines waveguide to improve the effective volume of the diamond, a sub-femtotesla sensitivity for AC field magnetometry can be achieved. The long-coherence high-density large-scale NVāˆ’ center ensemble in diamond means that types of room-temperature micro-sized solid-state quantum sensors with ultra-high sensitivity can be further developed in the near future.