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Quantum microwave-optical interface with nitrogen-vacancy centers in diamond

MetadataDetails
Publication Date2017-09-29
JournalPhysical review. A/Physical review, A
AuthorsBo Li, Fuli Li, Yuan Zhou, Sheng-li Ma, Fuli Li
InstitutionsXi’an Jiaotong University
Citations45
AnalysisFull AI Review Included

Technical Documentation & Analysis: Quantum Microwave-Optical Interface in Diamond

Section titled “Technical Documentation & Analysis: Quantum Microwave-Optical Interface in Diamond”

This document analyzes the research paper “Quantum microwave-optical interface with nitrogen-vacancy centers in diamond” (arXiv:1709.04852v1) to provide technical specifications and align the material requirements with 6CCVD’s advanced MPCVD diamond capabilities.


This research proposes a highly efficient, coherent quantum interface utilizing Nitrogen-Vacancy (NV) centers in diamond to bridge the gap between microwave and optical quantum domains.

  • Core Mechanism: An ensemble of NV centers embedded in diamond acts as a collective spin excitation mode ($\hat{b}$), mediating quantum state transfer between a microwave superconducting coplanar waveguide (CPW) cavity ($\hat{a}_1$) and an optical cavity ($\hat{a}_2$).
  • High Fidelity Protocols: Two conversion schemes are analyzed: a sequential Double-Swap protocol and an adiabatic Dark-State protocol (STIRAP-like).
  • Performance: Numerical simulations demonstrate high conversion fidelities, reaching up to 0.99 for coherent initial states under realistic decay conditions.
  • Robustness: The Dark-State scheme is shown to be extremely robust against collective spin dissipation ($\gamma_s$), as the conversion process evolves within a dark mode decoupled from the spin excitations.
  • Material Requirements: Experimental feasibility relies on high-quality diamond substrates hosting a dense, coherent NV ensemble ($1 \times 10^{12}$ centers) and operating at cryogenic temperatures (T $\sim$ 20 mK).
  • 6CCVD Value Proposition: Replication and extension of this work require ultra-high purity, low-strain Single Crystal Diamond (SCD) substrates, precisely polished and customized for integration with both microwave and optical resonators—a core specialization of 6CCVD.

The following hard data points and operational parameters are extracted from the analysis of the proposed hybrid quantum device:

ParameterValueUnitContext
NV Center Ensemble Density$1 \times 10^{12}$centersRequired for enhanced collective coupling ($\sqrt{N}g$)
Operating Temperature (T)$\sim 20$mKNecessary for negligible thermal photon occupation ($N_{1,2} \approx 0$)
Microwave CPW Cavity Q Factor$\sim 10^6$N/ARealistic quality factor for superconducting CPW
Optical Cavity Q Factor$\sim 10^9$N/AHigh Q factor (e.g., WGM or Fabry-Pérot)
Collective Coupling Strength (G)$\sim 2\pi \times 1$MHzEffective Raman transition rate ($G_1=G_2=G$)
Microwave Detuning ($\Delta_1$)$\sim 2\pi \times 200$MHzUsed for adiabatic elimination of excited states
Optical Detuning ($\Delta_2$)$\sim 2\pi \times 100$GHzUsed for adiabatic elimination of excited states
Microwave Decay Rate ($\kappa_1$)$0.003G$ ($\sim 2\pi \times 3$ kHz)N/A (or Hz)Realistic dissipation rate for CPW cavity
Collective Spin Decay Rate ($\gamma_s$)$0.01G$ ($\sim 2\pi \times 10$ kHz)N/A (or Hz)Based on demonstrated NV $T_2 > 100$ ”s
Optical Decay Rate ($\kappa_2$)$0.1G$ ($\sim 2\pi \times 100$ kHz)N/A (or Hz)Realistic dissipation rate for high-Q optical cavity
Maximum Conversion Fidelity0.99N/AAchieved for coherent state $

The proposed quantum interface relies on the following key steps and physical principles:

  1. Hybrid Setup Construction: The device integrates an ensemble of NV centers embedded in a diamond sample, placed simultaneously above a superconducting Coplanar Waveguide (CPW) resonator (microwave cavity $\hat{a}_1$) and coupled to an external optical cavity ($\hat{a}_2$).
  2. Four-Level System: The NV center is modeled as a four-level system, utilizing the 3A2 spin-1 ground state triplet ($|a\rangle, |b\rangle, |c\rangle$) and an excited optical state ($|e\rangle$).
  3. Raman Coupling: Quantum state transfer is achieved via two distinct Raman transitions driven by classical fields ($\Omega_1, \Omega_2$), coupling the NV spins to the microwave and optical cavity modes, respectively.
  4. Boson Mapping: Under the low excitation limit and large detuning conditions ($|\Delta_i| \gg |\Omega_i|, |g_i|$), the collective spin excitations of the NV ensemble are mapped onto a single bosonic mode ($\hat{b}$) using the Holstein-Primakoff representation.
  5. Effective Hamiltonian: The system dynamics are described by an effective beam-splitter Hamiltonian composed of two Jaynes-Cummings (JC) interactions, linking $\hat{a}_1 \leftrightarrow \hat{b}$ and $\hat{b} \leftrightarrow \hat{a}_2$.
  6. Dark-State Conversion (STIRAP): The adiabatic protocol modulates the coupling strengths $G_1(t)$ and $G_2(t)$ in a counterintuitive sequence, forcing the quantum state to evolve through a “spin dark mode” ($\hat{c}_d$) that is decoupled from the collective spin excitation mode ($\hat{b}$), thereby suppressing spin dissipation ($\gamma_s$).

Replicating or advancing this high-fidelity quantum interface requires diamond materials engineered to meet stringent quantum coherence, purity, and integration standards. 6CCVD is uniquely positioned to supply the necessary MPCVD diamond components.

Research Requirement6CCVD Material RecommendationTechnical Rationale
High Coherence & Low Strain (Essential for $T_2 > 100$ ”s)Optical Grade Single Crystal Diamond (SCD)Ultra-high purity MPCVD growth minimizes intrinsic defects and strain, providing the optimal host lattice for long-lived NV spin coherence.
High Density NV Ensemble (Requires controlled N content)Low-N SCD SubstratesStarting with high-purity, low-nitrogen SCD allows researchers to precisely control NV creation (via implantation/annealing) to achieve the required $1 \times 10^{12}$ center density without compromising coherence.

The integration of diamond into complex microwave (CPW) and optical cavity structures demands precise dimensional control and specialized surface preparation, which 6CCVD provides as standard services:

Integration Challenge6CCVD Customization CapabilitySpecification Range
CPW Resonator IntegrationCustom Metalization ServicesInternal deposition of Au, Pt, Pd, Ti, W, or Cu layers for direct integration with superconducting circuits.
Optical Cavity Coupling (WGM/Fabry-Pérot)Ultra-Precision PolishingSCD surfaces polished to $R_a < 1$ nm, minimizing optical scattering losses critical for achieving $Q \sim 10^9$ optical cavities.
Device Geometry & ThicknessCustom Dimensions and Thickness ControlSCD plates available from 0.1 ”m to 500 ”m thickness, and substrates up to 10 mm, with custom laser cutting for specific cavity footprints.
Large-Scale IntegrationLarge Area Polycrystalline Diamond (PCD)Wafers up to 125 mm (PCD) available for scaling up quantum device fabrication or thermal management applications.

6CCVD understands that material quality is paramount for achieving the high fidelities demonstrated in the Dark-State conversion protocol.

  • Expert Consultation: 6CCVD’s in-house PhD team specializes in diamond material science for quantum applications. We can assist researchers in selecting the optimal SCD purity, thickness, and surface orientation necessary to maximize NV yield and coherence time for similar Quantum Microwave-Optical Interface projects.
  • Global Supply Chain: We offer reliable global shipping (DDU default, DDP available) to ensure your critical materials arrive safely and promptly, regardless of your research location.

For custom specifications or material consultation, visit 6ccvd.com or contact our engineering team directly.

View Original Abstract

We propose an efficient scheme for a coherent quantum interface between microwave and optical photons using nitrogen-vacancy (NV) centers in diamond. In this setup, an NV center ensemble is simultaneously coupled to an optical and a microwave cavity. We show that, by using the collective spin excitation modes as an intermediary, quantum states can be transferred between the microwave cavity and the optical cavity through either a double-swap scheme or a dark-state protocol. This hybrid quantum interface may provide interesting applications in single microwave photon detections or quantum information processing.