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Hiding a Quantum Cache in Diamonds

MetadataDetails
Publication Date2016-06-22
JournalPhysics
AuthorsSimon C. Benjamin
InstitutionsUniversity of Oxford
Citations1
AnalysisFull AI Review Included

TECHNICAL DOCUMENTATION & ANALYSIS: Robust Quantum-Network Memory in Diamond NV Centers

Section titled “TECHNICAL DOCUMENTATION & ANALYSIS: Robust Quantum-Network Memory in Diamond NV Centers”

This documentation analyzes the key findings of the referenced paper, focusing on material requirements and providing tailored solutions from 6CCVD to accelerate quantum network research.

The research demonstrates a critical step toward realizing scalable quantum networks by creating a robust quantum memory node using Nitrogen-Vacancy (NV) centers in diamond.

  • Core Achievement: Storage of quantum coherence in a diamond-based node protected from noise induced by repeated, probabilistic remote entanglement attempts.
  • Material System: A single NV electronic spin hyperfine coupled to five individually controlled carbon-13 ($^{13}$C) nuclear spins used as memory qubits.
  • Decoherence Mitigation: Identified that memory fidelity was limited by dephasing induced during the stochastic electronic spin optical reset process after failed entanglement attempts.
  • Technical Solution: Quantum states were encoded into a Decoherence-Protected Subspace (DPS) utilizing two nuclear spins ($\vert\downarrow\uparrow\rangle$ and $\vert\uparrow\downarrow\rangle$ basis states) to effectively nullify the primary source of dephasing.
  • Performance Metric: The DPS memory demonstrated robustness, maintaining coherence for over 1000 repetitions of the noisy internode entangling protocol.
  • Significance: This finding paves the way for practical quantum repeaters and heralds the first demonstrations of remote entanglement purification using solid-state quantum nodes.

The following table summarizes the key experimental parameters and performance metrics extracted from the research paper.

ParameterValueUnitContext
Operating Temperature4KHelium bath cryostat
Applied Magnetic Field (B)40mTAlong NV symmetry axis
Electronic Spin Initialization Fidelity> 0.99N/APrior to experimental run
Nuclear Spin Control5N/AIndividually controlled $^{13}$C qubits
Nuclear Spin Coherence Time (T2*) Range4 to 19msMeasured for individual $^{13}$C spins
Parallel Hyperfine Coupling (A||) Range-48.7 to 21.2kHzRange across five observed $^{13}$C qubits
Optimal Decoupling Wait Time ($\tau$)$\approx 0.44$”sMinimizes dephasing due to singlet state decay
Fast Electronic Reset Time Scale (Minimum)29(1)nsUsing A1,2 transitions, high power
Metastable Singlet State Lifetime440nsDominates slow component of electronic reset
Coherence Decay Constant (Single Spin)$\approx 500$Repetitions (N)For spin with smallest coupling strength
Coherence Decay Constant (DPS Encoded Qubit)> 1000Repetitions (N)Using Decoherence-Protected Subspace

The experimental approach combines high-precision optical control, microwave manipulation, and robust material engineering within a cryogenic environment.

  1. Material Selection: Experiments were performed on a diamond device containing naturally abundant $^{13}$C nuclear spins, serving as the multiqubit register.
  2. Environmental Setup: The device was cooled to 4 K in a helium bath cryostat and subjected to a 40 mT magnetic field applied along the NV axis.
  3. Spin Initialization: The NV electronic spin ($m_s = 0$) was initialized using spin-selective optical transitions with fidelity > 0.99.
  4. Remote Entanglement Protocol: The Barrett-Kok sequence was employed, requiring repeated attempts due to probabilistic photon loss and inefficiency.
  5. Local Control: High-fidelity individual control of five surrounding $^{13}$C nuclear spins was achieved using tailored microwave pulse sequences, including BB1 composite pulses to suppress errors.
  6. Dynamic Decoupling: A dynamical decoupling sequence inherent in the entangling protocol was utilized, with the interval ($\tau$) optimized to $\approx 0.44$ ”s, matching the lifetime of the metastable singlet states.
  7. Decoherence Protection Strategy: Quantum states were stored in a Decoherence-Protected Subspace (DPS) formed by a symmetric superposition of two nuclear spins. This minimizes the effect of the linear precession frequency change ($\Delta\omega$) caused by electronic spin fluctuations.

This research highlights the absolute necessity of high-quality, customized MPCVD diamond for quantum applications. While the current work uses natural abundance material, 6CCVD can supply advanced, engineered SCD wafers that surpass current standards, enabling replication and acceleration of future research phases, such as full entanglement purification.

Research Requirement/Challenge6CCVD Material SolutionCustomization Potential
High Purity Host MaterialElectronic Grade SCD: Required to minimize native defects and ensure long, stable electronic spin coherence for the NV center.Guaranteed low nitrogen ([N]) and low substitutional nitrogen ([N$_{s}^0$]) concentrations.
Control of Nuclear Spin DensityIsotopically Engineered SCD: The paper relies on natural abundance $^{13}$C. To optimize memory performance, researchers require materials with either:Custom $^{13}$C enrichment percentages (e.g., 0.1% or 99.9%) or ultra-low $^{13}$C concentration (< 0.05 ppm) depending on the desired register size.
Enhanced Device IntegrationCustom Metalization Services: Future quantum repeater designs require integrated microwave/RF electrodes for rapid control pulses and deterministic operations.In-house deposition of Au, Pt, Ti, Cu, Pd, or W layers with precise alignment and patterning via laser cutting.
Reduced Decoherence (Surface Effects)Optical Grade SCD Polishing: Extremely flat surfaces are required to facilitate efficient optical coupling and stable laser addressing (Cryogenic operation).Ultra-smooth polishing down to Ra < 1 nm for Single Crystal Diamond (SCD) surfaces up to 10 mm thick.
Scalability and Custom Form FactorsCustom Dimensions and Thicknesses: As nodes scale up, unique substrate sizes become necessary for chip integration.SCD plates up to 500 ”m thick and custom substrate dimensions up to 10 mm thickness. PCD wafers available up to 125 mm diameter.

The robust quantum memory demonstrated here relies fundamentally on material selection that minimizes background noise while providing an addressable qubit register. 6CCVD’s in-house PhD team specializes in optimizing MPCVD growth recipes to deliver Isotopically Engineered SCD essential for replicating or extending this Quantum Network Memory research.

We offer detailed consultation on:

  • Selecting the ideal $^{13}$C concentration for desired nuclear spin coupling strength.
  • Specifying high-quality surfaces (Ra < 1 nm) critical for stable cryogenic optical interfaces.
  • Integrated metal layers necessary for microwave control sequences (e.g., Hermite pulse envelopes).

For custom specifications or material consultation, visit 6ccvd.com or contact our engineering team directly. We support global shipping (DDU default, DDP available).

View Original Abstract

The realization of a network of quantum registers is an outstanding challenge in quantum science and technology.We experimentally investigate a network node that consists of a single nitrogen-vacancy center electronic spin hyperfine coupled to nearby nuclear spins.We demonstrate individual control and readout of five nuclear spin qubits within one node.We then characterize the storage of quantum superpositions in individual nuclear spins under repeated application of a probabilistic optical internode entangling protocol.We find that the storage fidelity is limited by dephasing during the electronic spin reset after failed attempts.By encoding quantum states into a decoherence-protected subspace of two nuclear spins, we show that quantum coherence can be maintained for over 1000 repetitions of the remote entangling protocol.These results and insights pave the way towards remote entanglement purification and the realization of a quantum repeater using nitrogen-vacancy center quantum-network nodes.