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Proton Recoil Telescope Based on Diamond Detectors for the Measurement of Fusion Neutrons

MetadataDetails
Publication Date2016-05-24
JournalIEEE Transactions on Nuclear Science
AuthorsB. Caiffi, M. Osipenko, M. Ripani, M. Pillon, M. Taiuti
InstitutionsNational Agency for New Technologies, Energy and Sustainable Economic Development, Istituto Nazionale di Fisica Nucleare
Citations6
AnalysisFull AI Review Included

Technical Documentation & Analysis: MPCVD Diamond for Fusion Neutron Diagnostics

Section titled “Technical Documentation & Analysis: MPCVD Diamond for Fusion Neutron Diagnostics”

This research validates the use of segmented MPCVD diamond detectors in a Proton Recoil Telescope (PRT) configuration for high-resolution 14 MeV fusion neutron diagnostics, specifically addressing the harsh environment requirements of reactors like ITER.

  • Core Value Proposition: CVD diamond offers superior radiation hardness (43 eV displacement energy), high speed (2000 ”m2/(Vs) mobility), and low intrinsic noise due to its 5.5 eV bandgap, making it ideal for high-flux, high-temperature fusion environments.
  • Methodology: The PRT uses two aligned SCD crystals in coincidence, placed behind a plastic converter, to measure the energy of recoiled protons and effectively reject the large background from elastic neutron scattering on 12C nuclei.
  • Key Challenge Addressed: The ideal configuration (Prototype 1) requires ultra-thin SCD crystals (30 ”m) to achieve the lowest energy threshold (2 MeV spectrum reconstruction), a thickness currently difficult to source commercially.
  • 6CCVD Competitive Advantage: 6CCVD specializes in custom SCD fabrication, offering thicknesses down to 0.1 ”m, directly enabling the realization of the ideal Prototype 1 configuration necessary for optimal performance.
  • Performance Metrics: The tested prototype demonstrated an efficiency of 2.5 x 10-6 for 14 MeV neutrons and an energy resolution of 70 keV (fast chain readout).
  • Application: Critical technology for neutron spectrometry and monitoring structural damage/activation in next-generation fusion reactors (e.g., ITER).

The following table summarizes the critical material and performance parameters extracted from the study of the diamond-based proton recoil telescope prototypes.

ParameterValueUnitContext
Target Neutron Energy14MeVD-T Fusion Reaction
Required Operating TempHigh°CDiamond operates without cooling (5.5 eV bandgap)
Charge Carrier Mobility2000”m2/(Vs)Ensures fast charge collection (< few ns)
Diamond Band Gap5.5eVSuppresses dark current noise
Displacement Energy43eVHighest radiation hardness among neutron detectors
Ideal D1 Thickness (Prot. 1)30”mRequired for E > 2 MeV spectrum reconstruction
Ideal D2 Thickness (Prot. 1)700”mRequired to stop 14 MeV recoiled protons
Commercial D1 Thickness (Prot. 2)300”mLimits reconstruction threshold to E > 8 MeV
Crystal Area (Simulated)3 x 3mm2Sensitive volume dimensions
Converter MaterialPolyethylene (C2H4)N/AInduces (n,p) reaction
Converter Thickness20”mOptimized for conversion efficiency
Contact Thickness (Simulated)50nmCr contacts
Measured Efficiency (14 MeV)2.5 x 10-6N/ATested prototype (500/500 ”m crystals)
Energy Resolution (Fast Chain)70keVLimited by 11° solid angle aperture

The experimental approach focused on optimizing the geometry and material thicknesses of the segmented CVD diamond detector to maximize efficiency and background rejection for 14 MeV neutron spectrometry.

  1. Detector Configuration: The system was arranged as a Proton Recoil Telescope (PRT), consisting of a plastic (polyethylene) converter placed immediately in front of two sequential CVD diamond crystals (D1 and D2).
  2. Signal Generation: Incoming neutrons interact with the converter via the (n,p) reaction, generating recoiled protons. These protons pass through D1 (measuring dE/dx) and stop in D2 (measuring Etotal).
  3. Background Rejection: Fast coincidence measurements between D1 and D2 signals were used to reject background events, primarily those caused by elastic scattering of neutrons on the 12C atoms within the diamond crystals.
  4. Thickness Optimization (Simulation): Monte Carlo simulations (Geant4) were performed on three prototypes with varying SCD thicknesses (30/700 ”m, 300/500 ”m, 100/600 ”m) to determine the optimal configuration for achieving the lowest energy reconstruction threshold (down to 2 MeV).
  5. Prototype Assembly: A preliminary prototype was assembled using standard, commercially available electronic grade Single Crystal Diamond (SCD) detectors (500 ”m thick, 4.7 x 4.7 mm2 area) aligned 1.2 cm apart.
  6. Experimental Validation: Testing was conducted at the Frascati Neutron Generator (FNG) using 14 MeV neutrons generated by T(d,n)α fusion reactions, utilizing both charge sensitive (250 keV resolution) and fast (70 keV resolution) electronic readout chains.

This research highlights a critical need for highly customized, ultra-thin Single Crystal Diamond (SCD) materials to achieve optimal performance in fusion neutron diagnostics. 6CCVD is uniquely positioned to supply the necessary materials and fabrication services required to replicate and extend this research, particularly the ideal Prototype 1 configuration.

To achieve the low energy threshold (E > 2 MeV) and high resolution demonstrated in the simulations, the following 6CCVD materials are required:

Material SpecificationRequirement from Paper6CCVD CapabilityAdvantage
Single Crystal Diamond (SCD)Electronic Grade, High PurityHigh-quality SCD wafersSuperior charge collection and intrinsic noise suppression.
Custom Thickness (D1)30 ”m (Ideal Prototype 1)SCD available from 0.1 ”m to 500 ”mDirectly enables the ideal 30 ”m first crystal, which is currently unavailable commercially, allowing E > 2 MeV spectrum reconstruction.
Custom Thickness (D2)700 ”mSubstrates available up to 10 mmEasily meets the 700 ”m thickness requirement for stopping high-energy protons.
Polycrystalline Diamond (PCD)N/A (SCD preferred)Wafers up to 125 mmAvailable for large-area, lower-cost applications if SCD is not strictly required.

The success of the PRT design relies heavily on precise dimensions, specific thicknesses, and reliable electrical contacts. 6CCVD offers comprehensive customization services to meet these exact engineering requirements:

  • Precision Thickness Control: We can grow and polish SCD wafers to the exact optimized thicknesses (e.g., 30 ”m ± 5 ”m) required for the first detector (D1) to minimize the detection threshold.
  • Custom Dimensions and Segmentation: The paper utilized small 3 x 3 mm2 crystals. 6CCVD provides custom laser cutting and dicing to produce segmented detectors of any required size and geometry up to 125 mm wafers.
  • Advanced Metalization Services: The simulated prototypes used 50 nm Cr contacts. 6CCVD offers in-house metalization capabilities, including:
    • Standard Contacts: Au, Pt, Pd, Ti, W, Cu.
    • Custom Stacks: Fabrication of specific metal stacks (e.g., Ti/Pt/Au or custom Cr-based contacts) optimized for ohmic performance and harsh environment stability.
  • Surface Finish: SCD detectors require ultra-smooth surfaces for reliable thin-film contacts. 6CCVD guarantees Ra < 1 nm polishing for SCD, ensuring optimal electronic performance and bonding.

6CCVD’s in-house PhD team specializes in the material science and application engineering of CVD diamond. We provide expert consultation for projects requiring high-performance detectors in extreme environments.

  • Material Selection for Fusion Diagnostics: We assist researchers in selecting the optimal SCD grade (electronic vs. optical) and thickness profile necessary for similar fusion neutron spectrometry projects, ensuring the best balance between energy resolution, efficiency, and cost.
  • Design Optimization: We offer support in optimizing crystal geometry and metal contact design to minimize non-sensitive volumes and electronic noise, crucial for maximizing the signal-to-noise ratio in high-flux environments.

For custom specifications or material consultation, visit 6ccvd.com or contact our engineering team directly.

View Original Abstract

Diamonds are very promising candidates for the neutron diagnostics in harsh environments such as fusion reactors because of their proven radiation hardness. In comparison to the standard neutron diagnostics currently used (i.e., fission chambers, silicon based detectors, scintillators) CVD diamonds are less sensitive to $\gamma $ rays, which represents a huge background in fusion devices. Furthermore, their low leakage current provides a high energy resolution. A CVD diamond based detector has been proposed for the measurement of the 14 MeV neutrons from DT fusion reaction. The prototype was arranged in a proton recoil telescope configuration, featuring a plastic converter in front of the sensitive volume, in order to induce the (n, n) reactions which generate the recoil protons. The segmentation of the sensitive volume, achieved using two crystals with two dedicated electronic readouts, allowed to perform measurements in coincidence, which suppressed the neutron-carbon elastic scattering background. A preliminary prototype was assembled and tested at FNG (Frascati Neutron Generator), showing promising results regarding efficiency and energy resolution. © 2016 IEEE.

  1. 2003 - Geant4