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Experimental limits on the fidelity of adiabatic geometric phase gates in a single solid-state spin qubit

MetadataDetails
Publication Date2016-05-17
JournalNew Journal of Physics
AuthorsKai Zhang, Naufer Nusran, Bradley R. Slezak, Meenakshi Dutt
InstitutionsUniversity of Pittsburgh
Citations9
AnalysisFull AI Review Included

Technical Documentation: Geometric Phase Gates in NV Diamond

Section titled “Technical Documentation: Geometric Phase Gates in NV Diamond”

Analysis of Experimental Limits on Adiabatic Geometric Phase Gates in Solid-State Spin Qubits

Section titled “Analysis of Experimental Limits on Adiabatic Geometric Phase Gates in Solid-State Spin Qubits”

This document analyzes the requirements and findings of the research paper “Experimental limits on the fidelity of adiabatic geometric phase gates in a single solid-state spin qubit” (Zhang et al., 2016). It highlights how 6CCVD’s advanced MPCVD diamond materials and customization capabilities are essential for replicating and advancing this critical quantum information research.


  • Core Achievement: The study successfully measured the Berry phase and implemented an adiabatic geometric phase gate using a single Nitrogen-Vacancy (NV) center in a Type-IIa diamond substrate.
  • Fidelity Measurement: A high gate fidelity ($F_G = 0.978 \pm 0.026$) was achieved for a single $\pi/2$ phase shift gate operation.
  • Limiting Factor Identified: The decay in gate fidelity is primarily attributed to fast control field noise (fluctuations in the dynamic phase) occurring at frequencies higher than the spin echo clock frequency.
  • Material Requirement: The experiment relied on ultra-high purity, low-strain Single Crystal Diamond (SCD) to achieve a long environmental coherence time ($T_2 \sim 300$ ”s).
  • Methodology: Geometric manipulation was achieved via precise microwave control using an IQ modulator and Arbitrary Waveform Generator (AWG), coupled via a 20 ”m copper wire on the diamond surface.
  • 6CCVD Value Proposition: 6CCVD provides the necessary Optical Grade SCD substrates and custom metalization services required to minimize material-intrinsic noise and optimize microwave delivery for high-fidelity quantum control.

The following hard data points were extracted from the experimental results:

ParameterValueUnitContext
Diamond MaterialType-IIa SCDN/ABulk single crystal sample used for NV center
Crystal Orientation[1 1 1]N/AUsed for NV axis alignment
NV Ground State Splitting ($D$)2.87GHzZero magnetic field splitting
Static Bias Magnetic Field ($B_0$)$\approx 450$GaussApplied along the NV z-axis
Spin Echo Coherence Time ($T_2$)$\sim 300$”sEnvironmental limit without external control fields
Rabi Frequency ($\Omega$)12.5MHzUsed in amplitude scan experiments
Detuning ($\Delta$)10MHzUsed in Berry phase amplitude scan
$\pi/2$ Rotation Time$\sim 20$nsAchieved via microwave pulses
Gate Fidelity ($F_G$)$0.978 \pm 0.026$N/AMeasured fidelity for a single $\pi/2$ phase shift gate
Microwave Coupling20”mDiameter of copper wire placed on diamond surface
Decay Time Scale ($T_f$)2.2”sFitted decay time for long-time Rabi oscillation

The experiment utilized advanced quantum control techniques on a solid-state spin qubit:

  1. Qubit System Definition: A single NV center in a Type-IIa SCD sample was biased with a 450 Gauss DC magnetic field to create a pseudo-spin-1/2 qubit system ($|m_s = 0\rangle \leftrightarrow |m_s = -1\rangle$).
  2. Optical Control: Qubit initialization was performed via 532 nm laser excitation (optical pumping), and readout was achieved by measuring spin-dependent fluorescence (650-750 nm).
  3. Microwave Hamiltonian Control: Microwave radiation was delivered via a 20 ”m copper wire coupled to the diamond surface. The drive field was precisely modulated using an IQ modulator and an Arbitrary Waveform Generator (AWG).
  4. Adiabatic Circuit Generation: Fast amplitude and phase modulation were applied to the microwave drive field to create an effective rotating magnetic field, tracing a closed contour in parameter space to accumulate the geometric Berry phase.
  5. Noise Mitigation Technique: A resonant spin echo interferometry sequence was implemented to cancel the average dynamic phase and filter out slow environmental noise (extending $T_2$).
  6. Fidelity Analysis: Numerical simulations were performed, incorporating measured control field imperfections (e.g., single channel nonlinearity and amplitude imbalance in the IQ modulator), confirming that fast dynamic phase fluctuations limit gate fidelity.

6CCVD is uniquely positioned to supply the foundational materials and custom engineering required to replicate and extend this high-fidelity quantum control research. The paper’s findings underscore the necessity of minimizing both material-intrinsic noise and control-field imperfections—areas where 6CCVD excels.

To achieve the long coherence times ($T_2$) and high fidelity demonstrated, researchers require the highest quality diamond available.

Research Requirement6CCVD Material RecommendationTechnical Specification
Ultra-Low Defect Density (Type-IIa equivalent)Optical Grade Single Crystal Diamond (SCD)Nitrogen concentration < 1 ppb; extremely low strain and low substitutional defects, maximizing $T_2$.
High-Efficiency Qubit ReadoutOptical Grade SCDHigh transparency across the 532 nm excitation and 650-750 nm fluorescence windows.
Future Sensing/High-Power ApplicationsBoron-Doped Diamond (BDD) (If conductivity is required)Available for electrochemical or high-power microwave applications where grounding or charge dissipation is critical.

The experiment utilized a 20 ”m copper wire for microwave delivery, highlighting the need for precise integration of control electronics onto the diamond surface. 6CCVD offers comprehensive in-house engineering solutions:

  • Custom Metalization: We offer internal deposition and patterning of thin films, including Ti/Pt/Au (standard for quantum devices), Cu (as used in this study), Pd, and W. This capability allows researchers to integrate microstrip lines or coplanar waveguides directly onto the SCD substrate with high precision.
  • Precision Polishing: The paper noted systematic deviations due to imperfect driving waveforms (IQ modulator nonlinearity). Our Ra < 1 nm polishing for SCD ensures an atomically flat surface, minimizing surface defects that can interfere with metalization adhesion and microwave propagation uniformity.
  • Custom Dimensions: We provide SCD plates up to 500 ”m thick and PCD wafers up to 125 mm in diameter, cut to custom dimensions via laser processing, ensuring perfect fit for specialized quantum setups (e.g., confocal microscopy or cryogenic systems).

The research identified control field noise and imperfect driving waveforms (IQ modulator nonlinearity) as the primary limitations to gate fidelity.

  • Material Optimization for Noise Reduction: 6CCVD’s in-house PhD team specializes in material science for quantum applications. We assist clients in selecting the optimal SCD grade and thickness to mitigate environmental noise sources (e.g., surface spins, strain fields) that affect $T_2$ and $T_2$*.
  • Integration Consultation: We provide technical consultation on optimizing the interface between the diamond substrate and external control electronics (e.g., microwave antennas, electrodes) to minimize signal distortion and improve the fidelity of geometric quantum logic gates.

For custom specifications or material consultation, visit 6ccvd.com or contact our engineering team directly.

View Original Abstract

While it is often thought that the geometric phase is less sensitive to fluctuations in the control fields, a very general feature of adiabatic Hamiltonians is the unavoidable dynamic phase that accompanies the geometric phase. The effect of control field noise during adiabatic geometric quantum gate operations has not been probed experimentally, especially in the canonical spin qubit system that is of interest for quantum information. We present measurement of the Berry phase and carry out adiabatic geometric phase gate in a single solid-state spin qubit associated with the nitrogen-vacancy center in diamond. We manipulate the spin qubit geometrically by careful application of microwave radiation that creates an effective rotating magnetic field, and observe the resulting Berry phase signal via spin echo interferometry. Our results show that control field noise at frequencies higher than the spin echo clock frequency causes decay of the quantum phase, and degrades the fidelity of the geometric phase gate to the classical threshold after a few (~10) operations. This occurs in spite of the geometric nature of the state preparation, due to unavoidable dynamic contributions. In conclusion, we have carried out systematic analysis and numerical simulations to study the effects of the control field noise and imperfect driving waveforms on the quantum phase gate.